Magnetic properties of the triangular quantum spin tube [(CuCl2tachH)3Cl]Cl2 studied by NMR and magnetization

被引:6
|
作者
Furukawa, Yuji [1 ,2 ,3 ]
Sumida, Yuzuru [3 ]
Kumagai, Ken-ichi [3 ]
Borsa, Ferdinando [1 ,2 ,4 ]
Nojiri, Hiroyuki [5 ]
Shimizu, Yusei [3 ]
Amitsuka, Hiroshi [3 ]
Tenya, Ken-ichi [6 ]
Koegerler, Paul [1 ,2 ,7 ]
Cronin, Leroy [8 ]
机构
[1] Iowa State Univ, Ames Lab, Ames, IA 50011 USA
[2] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA
[3] Hokkaido Univ, Grad Sch Sci, Dept Phys, Sapporo, Hokkaido 0600810, Japan
[4] Univ Pavia, Dept Fis A Volta, I-27100 Pavia, Italy
[5] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan
[6] Shinshu Univ, Fac Educ, Dept Phys, Nagano 3808544, Japan
[7] Rhein Westfal TH Aachen, Inst Inorgan Chem, D-52074 Aachen, Germany
[8] Univ Glasgow, Dept Chem, Glasgow G12 8QQ, Lanark, Scotland
关键词
DYNAMICS;
D O I
10.1088/1742-6596/320/1/012047
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Static and dynamical properties of Cu2+ (3d(9); S = 1/2) spins in a twisted Heisenberg triangular spin tube, [(CuCl(2)tachH)(3)Cl]Cl-2, have been investigated by nuclear magnetic resonance (NMR) and magnetization measurements in the temperature range T = 0.05-300 K. Magnetization curves below 0.5 K show a clear change in slope around 5 T, attributed to a signature of 1/3 plateau in magnetization. From a systematic measurement of nuclear spin-lattice relaxation rates as a function of temperature and external field, the fluctuation frequency of Cu2+ spins is found to decrease with decreasing temperature, revealing an unusual slow spin dynamics at low temperatures.
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页数:6
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