Hot Carrier-Assisted Intrinsic Photoresponse in Graphene

被引:856
作者
Gabor, Nathaniel M. [1 ]
Song, Justin C. W. [1 ,2 ]
Ma, Qiong [1 ]
Nair, Nityan L. [1 ]
Taychatanapat, Thiti [1 ,3 ]
Watanabe, Kenji [4 ]
Taniguchi, Takashi [4 ]
Levitov, Leonid S. [1 ]
Jarillo-Herrero, Pablo [1 ]
机构
[1] MIT, Dept Phys, Cambridge, MA 02139 USA
[2] Harvard Univ, Harvard Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[3] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA
[4] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan
基金
美国国家科学基金会;
关键词
PHOTODETECTORS; GENERATION;
D O I
10.1126/science.1211384
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
We report on the intrinsic optoelectronic response of high-quality dual-gated monolayer and bilayer graphene p-n junction devices. Local laser excitation (of wavelength 850 nanometers) at the p-n interface leads to striking six-fold photovoltage patterns as a function of bottom-and top-gate voltages. These patterns, together with the measured spatial and density dependence of the photoresponse, provide strong evidence that nonlocal hot carrier transport, rather than the photovoltaic effect, dominates the intrinsic photoresponse in graphene. This regime, which features a long-lived and spatially distributed hot carrier population, may offer a path to hot carrier-assisted thermoelectric technologies for efficient solar energy harvesting.
引用
收藏
页码:648 / 652
页数:5
相关论文
共 28 条
  • [1] Ashcroft N., 2011, Solid State Physics
  • [2] Electronic Cooling in Graphene
    Bistritzer, R.
    MacDonald, A. H.
    [J]. PHYSICAL REVIEW LETTERS, 2009, 102 (20)
  • [3] Biased bilayer graphene: Semiconductor with a gap tunable by the electric field effect
    Castro, Eduardo V.
    Novoselov, K. S.
    Morozov, S. V.
    Peres, N. M. R.
    Dos Santos, J. M. B. Lopes
    Nilsson, Johan
    Guinea, F.
    Geim, A. K.
    Castro Neto, A. H.
    [J]. PHYSICAL REVIEW LETTERS, 2007, 99 (21)
  • [4] Thermopower and Nernst effect in graphene in a magnetic field
    Checkelsky, Joseph G.
    Ong, N. P.
    [J]. PHYSICAL REVIEW B, 2009, 80 (08)
  • [5] Extremely Efficient Multiple Electron-Hole Pair Generation in Carbon Nanotube Photodiodes
    Gabor, Nathaniel M.
    Zhong, Zhaohui
    Bosnick, Ken
    Park, Jiwoong
    McEuen, Paul L.
    [J]. SCIENCE, 2009, 325 (5946) : 1367 - 1371
  • [6] Transport measurements across a tunable potential barrier in graphene
    Huard, B.
    Sulpizio, J. A.
    Stander, N.
    Todd, K.
    Yang, B.
    Goldhaber-Gordon, D.
    [J]. PHYSICAL REVIEW LETTERS, 2007, 98 (23)
  • [7] Theory of thermopower in two-dimensional graphene
    Hwang, E. H.
    Rossi, E.
    Das Sarma, S.
    [J]. PHYSICAL REVIEW B, 2009, 80 (23):
  • [8] Kraemer D, 2011, NAT MATER, V10, P532, DOI [10.1038/NMAT3013, 10.1038/nmat3013]
  • [9] Contact and edge effects in graphene devices
    Lee, Eduardo J. H.
    Balasubramanian, Kannan
    Weitz, Ralf Thomas
    Burghard, Marko
    Kern, Klaus
    [J]. NATURE NANOTECHNOLOGY, 2008, 3 (08) : 486 - 490
  • [10] Lemme M. C., 2011, NANO LETT, DOI [10.1021/nl2019068, DOI 10.1021/NL2019068]