Visualization of charge ordering in a half-doped manganite by an electrostatic potential analysis

被引:14
作者
Kato, K. [1 ]
Moritomo, Y. [2 ]
Takata, M. [1 ,3 ]
Tanaka, H. [4 ]
Hamada, N. [5 ]
机构
[1] RIKEN, SPring Ctr 8, Wako, Saitama 6795148, Japan
[2] Univ Tsukuba, Dept Phys, Tsukuba, Ibaraki 3058571, Japan
[3] Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan
[4] Shimane Univ, Dept Mat Sci, Shimane 6908504, Japan
[5] Tokyo Univ Sci, Fac Sci & Technol, Noda, Chiba 2788510, Japan
关键词
D O I
10.1103/PhysRevB.77.081101
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have experimentally investigated the charge density distribution and the electrostatic potential for a charge-ordering doped manganite, Nd1/2Sr1/2MnO3. In the charge-ordered state, we observed a zigzag pattern of the charge density within the (010) plane. Judging from the MnO6 distortion, we ascribed the pattern to the bonding electron in the p(x(y))-d(x2-y2) hybridized state, not to the so-called d(3x)(2)-r(2)/d(3y2-r2) orbital ordering. We further calculated the electrostatic potential U(r) from the charge density and the atomic positions, which clearly indicates the checkerboard-type charge disproportionation within the (010) plane.
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页数:4
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