One-step catalytic conversion of ethanol into 1,3-butadiene using zinc-containing talc

被引:45
作者
Sekiguchi, Yasumasa [1 ,2 ]
Akiyama, Sohta [1 ]
Urakawa, Wataru [1 ]
Koyama, To-ru [1 ]
Miyaji, Akimitsu [1 ]
Motokura, Ken [1 ]
Baba, Toshihide [1 ]
机构
[1] Tokyo Inst Technol, Interdisciplinary Grad Sch Sci & Engn, Dept Environm Chem & Engn, Midori Ku, Yokohama, Kanagawa 2268502, Japan
[2] Press Kogyo Co Ltd, Kawasaki, Kanagawa 2108512, Japan
关键词
Ethanol; 1,3-Butadiene; Zinc-containing talc; High production rate; BUTADIENE FORMATION; SEPIOLITE;
D O I
10.1016/j.catcom.2015.04.023
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Compared with previously reported catalysts, zinc-containing talc exhibited the highest formation rate of 1,3-butadiene in one-step conversion of ethanol at 673 K. Our results showed that talc containing just 1.4 wt.% of ZnO produced 1,3-butadiene at a rate of 1.9 x 10(-2) mol g(-1) h(-1). (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:20 / 24
页数:5
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