Polarized emission in II-VI and perovskite colloidal quantum dots

被引:4
|
作者
Isarov, Maya [1 ]
Tan, Liang Z. [2 ]
Tilchin, Jenya [1 ]
Rabouw, Freddy T. [3 ]
Bodnarchuk, Maryna I. [4 ,5 ]
van Dijk-Moes, Relinde J. A. [3 ]
Carmi, Rotem [1 ]
Barak, Yahel [1 ]
Kostadinov, Alyssa [1 ]
Meir, Itay [1 ]
Vanmaekelbergh, Daniel [3 ]
Kovalenko, Maksym V. [4 ,5 ]
Rappe, Andrew M. [2 ]
Lifshitz, Efrat [1 ]
机构
[1] Technion, Solid State Inst, Russell Berrie Nanotechnol Inst, Schulich Fac Chem, IL-3200003 Haifa, Israel
[2] Univ Penn, Dept Chem, Philadelphia, PA 19104 USA
[3] Univ Utrecht, Debye Inst Nanomat Sci, Utrecht, Netherlands
[4] ETH, Dept Chem & Appl Biosci, Inst Inorgan Chem, Vladimir Prelog Weg 1, CH-8093 Zurich, Switzerland
[5] Empa Swiss Fed Labs Mat Sci & Technol, Lab Thin Films & Photovolta, Uberlandstr 129, CH-8600 Dubendorf, Switzerland
基金
欧盟地平线“2020”; 瑞士国家科学基金会; 欧洲研究理事会; 以色列科学基金会;
关键词
colloidal quantum dots; core/shell heterostructures; alloyed interfaces; blinking-free behavior; perovskites; magneto-optical properties; single dot spectroscopy; LEAD HALIDE PEROVSKITES; CORE-SHELL NANOCRYSTALS; SENSITIZED SOLAR-CELLS; SEMICONDUCTOR NANOCRYSTALS; PBSE/PBSEXS1-X CORE/SHELL; RADIATIVE RECOMBINATION; CARRIER MULTIPLICATION; INORGANIC PEROVSKITES; EXCHANGE INTERACTIONS; AUGER RECOMBINATION;
D O I
10.1088/1361-6455/aa8dd4
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The polarized emission of colloidal quantum dots from II-VI and perovskite semiconductors were investigated thoroughly, revealing information about the optical transitions in these materials and their potential use in various opto-electronic or spintronic applications. The studies included recording of the micro-photoluminescence of individual nanostructures at cryogenic temperatures, with or without the influence of an external magnetic field. The experimental conditions enabled detection of circular and/or linear polarized emission to elucidate the exciton manifolds, angular momentum of the emitting states, Lande g-factors, single exciton and biexciton binding energies, the excitons' effective Bohr radii, and the unique influence of the Rashba effect. The study advances the understanding of other phenomena such as electron-hole dissociation, long diffusion lengths, and spin coherence, facilitating appropriate design of optical and spin-based devices.
引用
收藏
页数:14
相关论文
共 50 条
  • [1] Room Temperature Colloidal Coating of II-VI Nanoplatelets with Quantum Dots
    Lifshitz, Efrat
    Horani, Faris
    Meir, Itay
    JOURNAL OF PHYSICAL CHEMISTRY C, 2021, 125 (46): : 25729 - 25738
  • [2] Design of cadmium-free colloidal II-VI semiconductor quantum dots exhibiting RGB emission
    Asano, Hiroshi
    Omata, Takahisa
    AIP ADVANCES, 2017, 7 (04):
  • [3] Very Low Threshold of Amplified Spontaneous Emission in II-VI Colloidal Quantum Dots at Low Exciton Number
    Dang, Cuong
    Nurmikko, A. V.
    2010 CONFERENCE ON LASERS AND ELECTRO-OPTICS (CLEO) AND QUANTUM ELECTRONICS AND LASER SCIENCE CONFERENCE (QELS), 2010,
  • [4] Surface Reconstructions in II-VI Quantum Dots
    Llusar, Jordi
    du Fosse, Indy
    Hens, Zeger
    Houtepen, Arjan
    Infante, Ivan
    ACS NANO, 2024, 18 (02) : 1563 - 1572
  • [5] II-VI quantum dots grown by MOVPE
    Suemune, I
    Yoshida, K
    Kumano, H
    Tawara, T
    Ueta, A
    Tanaka, S
    JOURNAL OF CRYSTAL GROWTH, 2003, 248 : 301 - 309
  • [6] DEPHASING PROCESSES IN II-VI QUANTUM DOTS
    WOGGON, U
    PORTUNE, M
    KLINGSHIRN, C
    GIESSEN, H
    FLUEGEL, B
    MOHS, G
    PEYGHAMBARIAN, N
    PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 1995, 188 (01): : 221 - 227
  • [7] Optical quantum control using II-VI quantum dots
    Henneberger, F
    Akimov, IA
    PHYSICA STATUS SOLIDI C - CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 3, NO 4, 2006, 3 (04): : 841 - +
  • [8] Optical Sensors Based on II-VI Quantum Dots
    Lesiak, Anna
    Drzozga, Kamila
    Cabaj, Joanna
    Banski, Mateusz
    Malecha, Karol
    Podhorodecki, Artur
    NANOMATERIALS, 2019, 9 (02)
  • [9] Enhanced spontaneous emission of CdSe quantum dots in monolithic II-VI pillar microcavities
    Lohmeyer, H.
    Kruse, C.
    Sebald, K.
    Gutowski, J.
    Hommel, D.
    APPLIED PHYSICS LETTERS, 2006, 89 (09)
  • [10] Preparation and characterization of overcoated II-VI quantum dots
    Xie, HY
    Liang, JG
    Liu, Y
    Zhang, ZL
    Pang, DW
    He, ZK
    Lu, ZX
    Huang, WH
    JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY, 2005, 5 (06) : 880 - 886