Fabrication and microstructure characterization of inert matrix fuel based on yttria stabilized zirconia

被引:20
作者
Hellwig, C [1 ]
Pouchon, M [1 ]
Restani, R [1 ]
Ingold, F [1 ]
Bart, G [1 ]
机构
[1] Paul Scherrer Inst, Nucl Energy & Safety Dept, CH-5232 Villigen, Switzerland
关键词
D O I
10.1016/j.jnucmat.2004.11.004
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The deployment of a suitable, Pu-bearing inert matrix fuel (IMF) could offer an attractive option as a single-recycling LWR strategy aimed at reducing the currently growing plutonium stockpiles. A development programme focusing on yttria stabilized zirconia (YSZ)-based IMF is conducted at PSI. YSZ-based IMF has so far been irradiated in two test reactors. The fabrication routes as well as the characterization of the irradiated material by ceramography, electronprobe microanalysis, and X-ray diffraction are presented. IMF fabrication by attrition milling of the oxide constituents is possible, but high sintering temperatures are required to achieve homogeneity. X-ray diffraction is a suitable tool to monitor the homogeneity. Extra efforts are needed to increase the density. (c) 2004 Elsevier B.V. All rights reserved.
引用
收藏
页码:163 / 170
页数:8
相关论文
共 21 条
[1]   A NEW FUEL MATERIAL FOR ONCE-THROUGH WEAPONS PLUTONIUM BURNING [J].
AKIE, H ;
MUROMURA, T ;
TAKANO, H ;
MATSUURA, S .
NUCLEAR TECHNOLOGY, 1994, 107 (02) :182-192
[2]   X-ray diffraction analysis and data interpretation of stabilized zirconia inert matrix fuel doped with plutonium [J].
Burghartz, M ;
Ledergerber, G ;
Ingold, F ;
Heimgartner, P ;
Degueldre, C .
PROGRESS IN NUCLEAR ENERGY, 2001, 38 (3-4) :247-250
[3]   Categorisation and priorities for future research on inert matrix fuels: An extended synthesis of the panel discussions [J].
Chawla, R ;
Konings, RJM .
PROGRESS IN NUCLEAR ENERGY, 2001, 38 (3-4) :455-458
[4]   Complex behavior in quaternary zirconias for inert matrix fuel: What do these materials look like at the nanometer scale? [J].
Conradson, SD ;
Degueldre, CA ;
Espinosa-Faller, FJ ;
Foltyn, SR ;
Sickafus, KE ;
Valdez, JA ;
Villella, PM .
PROGRESS IN NUCLEAR ENERGY, 2001, 38 (3-4) :221-230
[5]   Plutonium incineration in LWR's by a once-through cycle with a rock-like fuel [J].
Degueldre, C ;
Kasemeyer, U ;
Botta, F ;
Ledergerber, G .
SCIENTIFIC BASIS FOR NUCLEAR WASTE MANAGEMENT XIX, 1996, 412 :15-23
[6]   Inert matrix fuel performance during the first two irradiation cycles in a test reactor: comparison with modelling results [J].
Hellwig, C ;
Kasemeyer, U .
JOURNAL OF NUCLEAR MATERIALS, 2003, 319 :87-94
[7]   Interpretation of experimental results from moderate-power in-pile testing of a Pu-Er-Zr-oxide inert matrix fuel [J].
Hellwig, C ;
Kasemeyer, U ;
Ledergerber, G ;
Lee, BH ;
Lee, YW ;
Chawla, R .
ANNALS OF NUCLEAR ENERGY, 2003, 30 (03) :287-299
[8]   DIFFUSIVITIES OF FISSION-GAS SPECIES IN UO2 AND (U,GD)O-2 NUCLEAR-FUELS DURING IRRADIATION [J].
HIRAI, M ;
DAVIES, JH ;
WILLIAMSON, R .
JOURNAL OF NUCLEAR MATERIALS, 1995, 226 (1-2) :238-251
[9]   LATTICE-PARAMETERS AND DENSITY FOR Y2O3-STABILIZED ZRO2 [J].
INGEL, RP ;
LEWIS, D .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1986, 69 (04) :325-332
[10]   Comparison of pressurized water reactor core characteristics for 100% plutonium-containing loadings [J].
Kasemeyer, U ;
Paratte, JM ;
Grimm, P ;
Chawla, R .
NUCLEAR TECHNOLOGY, 1998, 122 (01) :52-63