Molecular imaging using recolliding electrons

被引:353
作者
Lein, Manfred
机构
[1] Univ Kassel, Ctr Interdisciplinary Nanostruct Sci & Technol, D-34132 Kassel, Germany
[2] Univ Kassel, Inst Phys, D-34132 Kassel, Germany
关键词
D O I
10.1088/0953-4075/40/16/R01
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
When molecules are subject to intense laser pulses, electrons can be detached, accelerated and driven back to the molecule, resulting in electron-ion recollisions. Recolliding electrons probe the structure and dynamics of molecules. We review the theoretical concepts and experimental achievements towards using recollisions to image molecules. We classify these methods by the choice of the observed signal, which can be one of high-harmonic radiation, electrons from high-order above-threshold ionization, or fragment kinetic energies from recollision-induced dissociation or Coulomb explosion. It is shown that sub-Angstrom and sub-femtosecond resolution is possible within these schemes.
引用
收藏
页码:R135 / R173
页数:39
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