An integrated biological-electrocatalytic process for highly-efficient treatment of coking wastewater

被引:36
作者
Wu, Zhen-Yu [1 ]
Zhu, Wei-Ping [1 ]
Liu, Yang [1 ]
Zhou, Lu-Lu [1 ]
Liu, Peng-Xi [1 ]
Xu, Juan [1 ,2 ]
机构
[1] East China Normal Univ, Sch Ecol & Environm Sci, Shanghai Key Lab Urban Ecol Proc & Ecorestorat, Zhejiang Tiantong Forest Ecosyst Natl Observat &, Shanghai, Peoples R China
[2] Inst Ecochongming IEC, 20 Cuiniao Rd, Shanghai 202162, Peoples R China
基金
中国国家自然科学基金;
关键词
Coking wastewater; Biological-electrocatalytic system; Three-dimensional biofilm electrode reactor; Biological aerated filter; REMOVAL; PERFORMANCE; REACTOR; NITROGEN; BIOFILM; SYSTEM; DENITRIFICATION; DEGRADATION; OZONATION; PRODUCTS;
D O I
10.1016/j.biortech.2021.125584
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
Coking wastewater is typically refractory, mainly due to its biological toxicity and complex composition. In this study, a novel integrated biological-electrocatalytic process consisting of two three-dimensional electrochemical reactors (3DERs), two biological aerated filters (BAFs), and a three-dimensional biofilm electrode reactor (3DBER) is developed for the advanced treatment of coking wastewater. 73.21% of chemical oxygen demand (COD), 38.02% of ammonium nitrogen (NH4+-N) and 91.46% of nitrate nitrogen (NO3--N) are removed by 3DERs. BAFs mainly convert NH4+-N to NO3--N through microbial nitrification. The 3DBER removes the residual NO3--N by bio-electrochemical denitrification. The integrated system can eliminate 74.72-83.27% of COD, 99.38-99.74% of NH4+-N, and 69.64-99.83% of total nitrogen from coking wastewater during the continuous operation, as well as significantly reducing the toxicity of the wastewater. The superiorities of the integrated 3DERs/BAFs/3DBER system recommend the application of such biological-electrocatalytic technology in the treatment of highly toxic wastewater.
引用
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页数:8
相关论文
共 43 条
[1]   Exploring the the relationship between the EPS property and the toxicity of sludge for treating 4-chlorophenol synthetic wastewater in a sequencing batch reactor [J].
Bao, Zheng ;
Chen, Xiurong ;
Zhao, Jianguo ;
Lin, Fengkai ;
Li, Jiahui ;
Zhang, Yuying .
INTERNATIONAL BIODETERIORATION & BIODEGRADATION, 2016, 110 :24-31
[2]   Advanced treatment of triazole fungicides discharged water in pilot scale by integrated system: Enhanced electrochemical oxidation, upflow biological aerated filter and electrodialysis [J].
Cui, Tao ;
Zhang, Yonghao ;
Han, Weiqing ;
Li, Jiansheng ;
Sun, Xiuyun ;
Shen, Jinyou ;
Wang, Lianjun .
CHEMICAL ENGINEERING JOURNAL, 2017, 315 :335-344
[3]  
Deng Y, CHEM ENG J, V424
[4]   Treatment of organic wastewater containing nitrogen and chlorine by combinatorial electrochemical system: Taking biologically treated landfill leachate treatment as an example [J].
Deng, Yang ;
Chen, Nan ;
Feng, Chuanping ;
Chen, Fangxin ;
Wang, Haishuang ;
Kuang, Peijing ;
Feng, Zhengyuan ;
Liu, Tong ;
Gao, Yu ;
Hu, Weiwu .
CHEMICAL ENGINEERING JOURNAL, 2019, 364 :349-360
[5]   Synergistic effects of electricity and biofilm on Rhodamine B (RhB) degradation in three-dimensional biofilm electrode reactors (3D-BERs) [J].
Feng, Lei ;
Li, Xiu-yan ;
Gan, Li-hong ;
Xu, Juan .
ELECTROCHIMICA ACTA, 2018, 290 :165-175
[6]   Electrochemical oxidation of humic acid and sanitary landfill leachate: Influence of anode material, chloride concentration and current density [J].
Fernandes, A. ;
Santos, D. ;
Pacheco, M. J. ;
Ciriaco, L. ;
Lopes, A. .
SCIENCE OF THE TOTAL ENVIRONMENT, 2016, 541 :282-291
[7]   Removal and transformation of polycyclic aromatic hydrocarbons during electrocoagulation treatment of an industrial wastewater [J].
Gong, Chenhao ;
Shen, Gang ;
Huang, Haiou ;
He, Peiran ;
Zhang, Zhongguo ;
Ma, Baoqing .
CHEMOSPHERE, 2017, 168 :58-64
[8]   Denitrification of simulated municipal wastewater treatment plant effluent using a three-dimensional biofilm-electrode reactor: Operating performance and bacterial community [J].
Hao, Ruixia ;
Li, Sumei ;
Li, Jianbing ;
Meng, Chengcheng .
BIORESOURCE TECHNOLOGY, 2013, 143 :178-186
[9]   Microbial interspecific interaction and nitrogen metabolism pathway for the treatment of municipal wastewater by iron carbon based constructed wetland [J].
Huang, Xiao ;
Yang, Xinmei ;
Zhu, Jia ;
Yu, Jianghua .
BIORESOURCE TECHNOLOGY, 2020, 315
[10]   Multiple response optimization for high efficiency energy saving treatment of rhodamine B wastewater in a three-dimensional electrochemical reactor [J].
Ji, Jing ;
Liu, Yang ;
Yang, Xue-yuan ;
Xu, Juan ;
Li, Xiu-yan .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2018, 218 :300-308