Preparation and photoelectrochemical performance of porous TiO2/graphene nanocomposite films

被引:10
作者
Chien Nguyen Van [1 ]
Nguyen Thanh Hai [2 ]
Olejnicek, Jiri [3 ]
Ksirova, Petra [3 ]
Kohout, Michal [3 ]
Dvorakova, Michaela [3 ]
Pham Van Hao [1 ]
Phan Ngoc Hong [1 ]
Manh Cuong Tran [4 ]
Do Hoang Tung [5 ]
Dang Van Thanh [2 ,6 ]
机构
[1] Vietnam Acad Sci & Technol, Inst Mat & Sci, Hanoi, Vietnam
[2] Res & Dev Ctr Adv Technol, 107 Dao Tan Rd, Hanoi, Vietnam
[3] Czech Acad Sci, Inst Phys, Prague, Czech Republic
[4] Hanoi Natl Univ Educ, Fac Phys, Hanoi, Vietnam
[5] Vietnam Acad Sci & Technol, Inst Phys, Hanoi, Vietnam
[6] Univ Med & Pharm, TNU, Thai Nguyen City, Vietnam
关键词
Porous structure; TiO2/graphene nanocomposite; Photoelectrochemical water splitting; SOLAR-CELLS; GRAPHENE; NANOPARTICLES;
D O I
10.1016/j.matlet.2017.11.008
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Direct photoelectrochemical (PEC) water splitting using solar energy offers a potential pathway to produce a clean, renewable, and sustainable source of hydrogen fuel. Herein, the TiO2/graphene nanocomposite for PEC water splitting was prepared by a combination of the drop-cast deposition of graphene nanosheets and the sputtering deposition of TiO2 films. The surface morphology, crystalline phase, and optical properties were investigated by Scanning electron microscopy, Raman spectroscopy, and Ultraviolet-visible spectroscopy. The results showed that the thermal treatment process and the combination with graphene nanosheets could effectively enhance PEC water oxidation of TiO2 photocatalyst. This enhancement could attribute to efficient charge transfer from TiO2 to graphene and the porous graphene framework. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:109 / 113
页数:5
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