Pulsed laser deposition of antimony selenosulfide thin film for efficient solar cells

被引：26

作者：

Chen, Chao ^{[1
]}

Yin, Yiwei ^{[1
]}

Lian, Weitao ^{[1
]}

Jiang, Lifeng ^{[1
]}

Tang, Rongfeng ^{[1
]}

Jiang, Chenhui ^{[1
]}

Wu, Chunyan ^{[1
]}

Gao, Di ^{[1
]}

Wang, Xiaomin ^{[1
]}

Fang, Fang ^{[1
]}

Zhu, Changfei ^{[1
]}

Chen, Tao ^{[1
]}

机构：

[1] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei Natl Lab Phys Sci Microscale, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China

来源：

APPLIED PHYSICS LETTERS | 2020年 / 116卷 / 13期

基金：

中国国家自然科学基金;

关键词：

SB2S3; FILM; EVAPORATION;

D O I：

10.1063/1.5139467

中图分类号：

O59 [应用物理学];

学科分类号：

摘要：

Antimony selenosulfide, Sb-2(SxSe1-x)(3), has been considered as a promising light harvesting material for low-cost, non-toxic, and stable solar cell applications. However, current preparation methods of Sb-2(SxSe1-x)(3) suffer from low-quality films, which hampers the performance improvement in Sb-2(SxSe1-x)(3)-based solar cells. Herein, we develop a pulsed laser deposition technique to fabricate antimony selenosulfide films with flat and compact surface morphology and high crystallinity. The composition of the as-obtained films can be conveniently tuned via varying molar ratios of Sb2S3 and Se in targets. At optimized conditions, we fabricate planar heterojunction solar cells and then obtain a significantly improved power conversion efficiency of 7.05%. Our research offers a facile and robust preparation method for Sb-2(SxSe1-x)(3) films with enhanced photovoltaic properties. Published under license by AIP Publishing.

引用

页数：4

共 28 条

[1] Influence of the electron buffer layer on the photovoltaic performance of planar Sb2(SxSe1-x)3 solar cells [J].

Andres Jaramillo-Quintero, Oscar ;

Elizabeth Rincon, Marina ;

Vasquez-Garcia, Geovanni ;

Nair, P. K. .

PROGRESS IN PHOTOVOLTAICS, 2018, 26 (09) :709-717

[2]

[Anonymous], 2019, INTEL 64 IA 32 ARCHI, V3, DOI DOI 10.1002/SOLR.201800280

[3]

[Anonymous], 2014, CANCER DISCOV, V4, pOF5, DOI DOI 10.1002/AENM.201301680

[4] Characterization of basic physical properties of Sb2Se3 and its relevance for photovoltaics [J].

Chen C. ;

Bobela D.C. ;

Yang Y. ;

Lu S. ;

Zeng K. ;

Ge C. ;

Yang B. ;

Gao L. ;

Zhao Y. ;

Beard M.C. ;

Tang J. .

Frontiers of Optoelectronics, 2017, 10 (01) :18-30

[5] Deep centers in a CuInGaSe2/CdS/ZnO:B solar cell [J].

Choi, In-Hwan ;

Choi, Chul-Hwan ;

Lee, Joo-Won .

PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE, 2012, 209 (06) :1192-1197

[6] Highly Improved Sb2S3 Sensitized-Inorganic-Organic Heterojunction Solar Cells and Quantification of Traps by Deep-Level Transient Spectroscopy [J].

Choi, Yong Chan ;

Lee, Dong Uk ;

Noh, Jun Hong ;

Kim, Eun Kyu ;

Seok, Sang Il .

ADVANCED FUNCTIONAL MATERIALS, 2014, 24 (23) :3587-3592

[7] High-throughput method to deposit continuous composition spread Sb2(SexS1 - x)3 thin film for photovoltaic application [J].

Deng, Hui ;

Yuan, Shengjie ;

Yang, Xiaokun ;

Zhang, Jian ;

Khan, Jahangeer ;

Zhao, Yang ;

Ishaq, Muhammad ;

Ye, Wanneng ;

Cheng, Yi-Bing ;

Song, Haisheng ;

Tang, Jiang .

PROGRESS IN PHOTOVOLTAICS, 2018, 26 (04) :281-290

[8] Interpretation of admittance, capacitance-voltage, and current-voltage signatures in Cu(In,Ga)Se2 thin film solar cells [J].

Eisenbarth, Tobias ;

Unold, Thomas ;

Caballero, Raquel ;

Kaufmann, Christian A. ;

Schock, Hans-Werner .

JOURNAL OF APPLIED PHYSICS, 2010, 107 (03)

[9] High Open Circuit Voltage in Sb2S3/Metal Oxide-Based Solar Cells [J].

Englman, Tzofia ;

Terkieltaub, Eyal ;

Etgar, Lioz .

JOURNAL OF PHYSICAL CHEMISTRY C, 2015, 119 (23) :12904-12909

[10] Sb2(SxSe1-x)3 sensitized solar cells prepared by solution deposition methods [J].

Hernandez-Granados, Araceli ;

Escorcia-Garcia, Jose ;

Perez-Martinez, Diego ;

Garcia-Cerrillo, Jose ;

Menchaca-Campos, Carmina ;

Hu, Hailin .

MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING, 2016, 56 :222-227

← 1 2 3 →