Fourier transform two-dimensional electronic-vibrational spectroscopy using an octave-spanning mid-IR probe

被引：41
|
作者：
Gaynor, James D. [1 ]
Courtney, Trevor L. [1 ]
Balasubramanian, Madhumitha [1 ]
Khalil, Munira [1 ]
机构：
[1] Univ Washington, Dept Chem, Seattle, WA 98195 USA
来源：
OPTICS LETTERS | 2016年 / 41卷 / 12期
基金：
美国国家科学基金会;
关键词：
ULTRAVIOLET; DYNAMICS; PULSES; MOTION; SHOT;
D O I：
10.1364/OL.41.002895
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
The development of coherent Fourier transform two-dimensional electronic-vibrational (2D EV) spectroscopy with acousto-optic pulse-shaper-generated near-UV pump pulses and an octave-spanning broadband mid-IR probe pulse is detailed. A 2D EV spectrum of a silicon wafer demonstrates the full experimental capability of this experiment, and a 2D EV spectrum of dissolved hexacyanoferrate establishes the viability of our 2D EV experiment for studying condensed phase molecular ensembles. (C) 2016 Optical Society of America
引用
收藏
页码：2895 / 2898
页数：4
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