A review of N-functionalized solid adsorbents for post-combustion CO2 capture

被引：217

作者：

Hu, Xiayi ^{[1
,2
]}

Liu, Libin ^{[1
]}

Luo, Xiao ^{[3
]}

Xiao, Gongkui ^{[4
]}

Shiko, Elenica ^{[5
]}

Zhang, Rui ^{[1
]}

Fan, Xianfeng ^{[2
]}

Zhou, Yefeng ^{[1
]}

Liu, Yang ^{[6
]}

Zeng, Zhaogang ^{[7
]}

Li, Chao'en ^{[8
]}

机构：

[1] Xiangtan Univ, Coll Chem Engn, Xiangtan 411105, Peoples R China

[2] Univ Edinburgh, Inst Mat & Proc, Sch Engn, Mayfield Rd, Edinburgh EH9 3JL, Midlothian, Scotland

[3] Hunan Univ, Coll Chem & Chem Engn, Changsha 410082, Hunan, Peoples R China

[4] Univ Western Australia, Dept Chem Engn, 35 Stirling Hwy, Crawley, WA 6009, Australia

[5] Univ Bath, Dept Chem Engn, Bath BA2 7AY, Avon, England

[6] Hunan BG Wellpoint Environm Sci & Technol Co Ltd, Changsha 41000, Peoples R China

[7] Xiangtan Sepiolite Technol Co Ltd, Xiangtan 411100, Peoples R China

[8] CSIRO Energy, 71 Normanby Rd, Clayton North, Vic 3169, Australia

来源：

APPLIED ENERGY | 2020年 / 260卷

基金：

中国国家自然科学基金;

关键词：

NFSAs; CO2; capture; Functionalization; Amine; Solid porous-based materials; Adsorption performance; CARBON-DIOXIDE CAPTURE; DOPED POROUS CARBON; MESOPOROUS MOLECULAR-SIEVE; MODIFIED ZEOLITE 13X; ADSORPTION PERFORMANCE; ACTIVATED CARBON; FLUE-GAS; SUPPORTED POLYETHYLENIMINE; OXIDATIVE-DEGRADATION; SELECTIVE ADSORPTION;

D O I：

10.1016/j.apenergy.2019.114244

中图分类号：

TE [石油、天然气工业]; TK [能源与动力工程];

学科分类号：

0807 ; 0820 ;

摘要：

Over the past decade, amine-loaded solid adsorbents for capturing CO2 from power plants have been widely studied. Various nitrogen (N) sources have been used for this purpose, and the current range of adsorbents, referred to here as N-functionalized solid adsorbent (NFSAs), are the subject of this review. The main synthesis methods of NFSAs are described and recent progress in the field discussed. Criteria for improving NFSA performance are highlighted with reference to a variety of solid supports, providing guidance on the selection of highly efficient, inexpensive adsorbents. A thorough assessment of adsorption mechanisms and factors influencing the adsorption process is given. The review concludes by exploring future research and development opportunities, as well as pathways for commercializing NFSAs.

引用

页数：18

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