White Light-Emitting Diodes Based on Individual Polymerized Carbon Nanodots

被引:38
作者
Xie, Zheng [1 ]
Yin, Zhengmao [2 ,3 ]
Wu, Yongzhong [2 ]
Liu, Chunyan [1 ]
Hao, Xiaopeng [2 ]
Du, Qingqing [1 ,2 ]
Xu, Xiangang [2 ,4 ]
机构
[1] Chinese Acad Sci, Tech Inst Phys & Chem, Lab Photochem Convers & Optoelect Mat, 29 Zhongguancun East Rd, Beijing 100190, Peoples R China
[2] Shandong Univ, State Key Lab Crystal Mat, 27 Shandanan Rd, Jinan 250100, Peoples R China
[3] Qingdao Univ Sci & Technol, Coll Mat Sci & Engn, Qingdao 266042, Peoples R China
[4] Shandong Inspur HuaGuang Optoelect CO LTD, 1835 Tianchen St, Jinan 250101, Shandong, Peoples R China
来源
SCIENTIFIC REPORTS | 2017年 / 7卷
基金
中国国家自然科学基金;
关键词
GRAPHENE QUANTUM DOTS; FULL-COLOR EMISSION; ONE-POT SYNTHESIS; PHOTOLUMINESCENCE; NANOPARTICLES; NANOCRYSTALS; PERFORMANCE; NANOCOMPOSITE; COMPOSITES; EFFICIENT;
D O I
10.1038/s41598-017-12083-2
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
A search for new phosphor materials that exhibit high light-emission, spectral purity, long-time stability and processability capture particular attention to modern solid-state lighting. Here, polymerizable silane pre-functionalized carbon dot (SiCD) fluids were dripped and co-polymerized or completely bulk polymerized to build color conversion and encapsulation coatings of commercially available GaN blue LEDs. Most parameters of SiCD-based white LEDs were similar to or even better than those of phosphor-based white LEDs, particularly the insensitivity to excitation wavelength and working current. Thus, SiCDs were superior to those phosphors in terms of broadband properties, high transparency (no light blocking and leaking), as well as arbitrary doping of its content as color conversion and encapsulation layers simultaneously, unique solubility,
引用
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页数:9
相关论文
共 68 条
[1]   Luminescent Carbon Nanodots: Emergent Nanolights [J].
Baker, Sheila N. ;
Baker, Gary A. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (38) :6726-6744
[2]   Photoluminescence-Tunable Carbon Nanodots: Surface-State Energy-Gap Tuning [J].
Bao, Lei ;
Liu, Cui ;
Zhang, Zhi-Ling ;
Pang, Dai-Wen .
ADVANCED MATERIALS, 2015, 27 (10) :1663-+
[3]   Quantum dots go on display [J].
Bourzac, Katherine .
NATURE, 2013, 493 (7432) :283-283
[4]   Photoluminescent organosilane-functionalized carbon dots as temperature probes [J].
Chen, Po-Cheng ;
Chen, Ya-Na ;
Hsu, Pin-Che ;
Shih, Chung-Chien ;
Chang, Huan-Tsung .
CHEMICAL COMMUNICATIONS, 2013, 49 (16) :1639-1641
[5]   High-Efficiency Silicon Nanocrystal Light-Emitting Devices [J].
Cheng, Kai-Yuan ;
Anthony, Rebecca ;
Kortshagen, Uwe R. ;
Holmes, Russell J. .
NANO LETTERS, 2011, 11 (05) :1952-1956
[6]   Hybrid Silicon Nanocrystal-Organic Light-Emitting Devices for Infrared Electroluminescence [J].
Cheng, Kai-Yuan ;
Anthony, Rebecca ;
Kortshagen, Uwe R. ;
Holmes, Russell J. .
NANO LETTERS, 2010, 10 (04) :1154-1157
[7]  
Choi H, 2013, NAT PHOTONICS, V7, P732, DOI [10.1038/nphoton.2013.181, 10.1038/NPHOTON.2013.181]
[8]   Solution-processed, high-performance light-emitting diodes based on quantum dots [J].
Dai, Xingliang ;
Zhang, Zhenxing ;
Jin, Yizheng ;
Niu, Yuan ;
Cao, Hujia ;
Liang, Xiaoyong ;
Chen, Liwei ;
Wang, Jianpu ;
Peng, Xiaogang .
NATURE, 2014, 515 (7525) :96-99
[9]   Quantum dot integrated LEDs using photonic and excitonic color conversion [J].
Demir, Hilmi Volkan ;
Nizamoglu, Sedat ;
Erdem, Talha ;
Mutlugun, Evren ;
Gaponik, Nikolai ;
Eychmueller, Alexander .
NANO TODAY, 2011, 6 (06) :632-647
[10]   Functional Surface Engineering of C-Dots for Fluorescent Biosensing and in Vivo Bioimaging [J].
Ding, Changqin ;
Zhu, Anwei ;
Tian, Yang .
ACCOUNTS OF CHEMICAL RESEARCH, 2014, 47 (01) :20-30