Delay in recovery of the Antarctic ozone hole from unexpected CFC-11 emissions

被引:58
作者
Dhomse, S. S. [1 ,2 ]
Feng, W. [1 ,3 ]
Montzka, S. A. [4 ]
Hossaini, R. [5 ]
Keeble, J. [6 ,7 ]
Pyle, J. A. [6 ,7 ]
Daniel, J. S. [4 ]
Chipperfield, M. P. [1 ,2 ]
机构
[1] Univ Leeds, Sch Earth & Environm, Leeds LS2 9JT, W Yorkshire, England
[2] Univ Leeds, NCEO, Leeds LS2 9JT, W Yorkshire, England
[3] Univ Leeds, NCAS, Leeds LS2 9JT, W Yorkshire, England
[4] NOAA, Earth Syst Res Lab, Global Monitoring Div, Boulder, CO USA
[5] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England
[6] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England
[7] Univ Cambridge, NCAS, Cambridge CB2 1EW, England
基金
英国自然环境研究理事会;
关键词
CHEMICAL-TRANSPORT MODEL; STRATOSPHERIC OZONE; SOUTHERN-HEMISPHERE; RETURN DATES; CHEMISTRY; INCREASE; EMERGENCE; DEPLETION; VERSION; IMPACT;
D O I
10.1038/s41467-019-13717-x
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The Antarctic ozone hole is decreasing in size but this recovery will be affected by atmospheric variability and any unexpected changes in chlorinated source gas emissions. Here, using model simulations, we show that the ozone hole will largely cease to occur by 2065 given compliance with the Montreal Protocol. If the unusual meteorology of 2002 is repeated, an ozone-hole-free-year could occur as soon as the early 2020s by some metrics. The recently discovered increase in CFC-11 emissions of similar to 13 Gg yr(-1) may delay recovery. So far the impact on ozone is small, but if these emissions indicate production for foam use much more CFC-11 may be leaked in the future. Assuming such production over 10 years, disappearance of the ozone hole will be delayed by a few years, although there are significant uncertainties. Continued, substantial future CFC-11 emissions of 67 Gg yr(-1) would delay Antarctic ozone recovery by well over a decade.
引用
收藏
页数:12
相关论文
共 49 条
[41]   Current sources of carbon tetrachloride (CCl4) in our atmosphere [J].
Sherry, David ;
McCulloch, Archie ;
Liang, Qing ;
Reimann, Stefan ;
Newman, Paul A. .
ENVIRONMENTAL RESEARCH LETTERS, 2018, 13 (02)
[42]   ECMWF analyses and forecasts of stratospheric winter polar vortex breakup: September 2002 in the Southern Hemisphere and related events [J].
Simmons, A ;
Hortal, M ;
Kelly, G ;
McNally, A ;
Untch, A ;
Uppala, S .
JOURNAL OF THE ATMOSPHERIC SCIENCES, 2005, 62 (03) :668-689
[43]   Stratospheric ozone depletion: A review of concepts and history [J].
Solomon, S .
REVIEWS OF GEOPHYSICS, 1999, 37 (03) :275-316
[44]   Emergence of healing in the Antarctic ozone layer [J].
Solomon, Susan ;
Ivy, Diane J. ;
Kinnison, Doug ;
Mills, Michael J. ;
Neely, Ryan R., III ;
Schmidt, Anja .
SCIENCE, 2016, 353 (6296) :269-274
[45]   Decline in Antarctic Ozone Depletion and Lower Stratospheric Chlorine Determined From Aura Microwave Limb Sounder Observations [J].
Strahan, Susan E. ;
Douglass, Anne R. .
GEOPHYSICAL RESEARCH LETTERS, 2018, 45 (01) :382-390
[46]   The Earth Observing System Microwave Limb Sounder (EOS MLS) on the Aura satellite [J].
Waters, JW ;
Froidevaux, L ;
Harwood, RS ;
Jarnot, RF ;
Pickett, HM ;
Read, WG ;
Siegel, PH ;
Cofield, RE ;
Filipiak, MJ ;
Flower, DA ;
Holden, JR ;
Lau, GKK ;
Livesey, NJ ;
Manney, GL ;
Pumphrey, HC ;
Santee, ML ;
Wu, DL ;
Cuddy, DT ;
Lay, RR ;
Loo, MS ;
Perun, VS ;
Schwartz, MJ ;
Stek, PC ;
Thurstans, RP ;
Boyles, MA ;
Chandra, KM ;
Chavez, MC ;
Chen, GS ;
Chudasama, BV ;
Dodge, R ;
Fuller, RA ;
Girard, MA ;
Jiang, JH ;
Jiang, YB ;
Knosp, BW ;
LaBelle, RC ;
Lam, JC ;
Lee, KA ;
Miller, D ;
Oswald, JE ;
Patel, NC ;
Pukala, DM ;
Quintero, O ;
Scaff, DM ;
Van Snyder, W ;
Tope, MC ;
Wagner, PA ;
Walch, MJ .
IEEE TRANSACTIONS ON GEOSCIENCE AND REMOTE SENSING, 2006, 44 (05) :1075-1092
[47]   Age of stratospheric air: Theory, observations, and models [J].
Waugh, DW ;
Hall, TM .
REVIEWS OF GEOPHYSICS, 2002, 40 (04) :1-1
[48]   Total ozone trends from 1979 to 2016 derived from five merged observational datasets - the emergence into ozone recovery [J].
Weber, Mark ;
Coldewey-Egbers, Melanie ;
Fioletov, Vitali E. ;
Frith, Stacey M. ;
Wild, Jeannette D. ;
Burrows, John P. ;
Long, Craig S. ;
Loyola, Diego .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2018, 18 (03) :2097-2117
[49]  
WMO, 2018, 58 WMO GLOB OZ RES M