Polyimide-based composite coatings for simultaneously enhanced mechanical and tribological properties by polyhedral oligomeric silsesquioxane

被引:13
作者
Yu, Chuanyong [1 ]
Liao, Yuwen [1 ]
Zhang, Peng [1 ,2 ]
Li, Bin [3 ]
Li, Shuangjian [1 ,2 ]
Wang, Qiwei [1 ,2 ]
Li, Wei [1 ,2 ]
机构
[1] Jinan Univ, Inst Adv Wear & Corros Resistant & Funct Mat, Guangzhou 510632, Peoples R China
[2] Jinan Univ, Shaoguan Res Inst, Shaoguan 512027, Peoples R China
[3] Southern Univ Sci & Technol, Dept Mat Sci & Engn, Guangdong Prov Key Lab Funct Oxide Mat & Devices, Shenzhen 518055, Peoples R China
基金
中国国家自然科学基金;
关键词
Polyimide; Polyhedral oligomeric silsesquioxane; Lubrication coating; Mechanical properties; Organic-inorganic hybrid; SURFACE-PROPERTIES; POSS; NANOCOMPOSITES; WEAR; FILM; TRIBOCHEMISTRY; PERFORMANCE; BEHAVIORS;
D O I
10.1016/j.triboint.2022.107521
中图分类号
TH [机械、仪表工业];
学科分类号
0802 ;
摘要
The increasingly harsh service condition of lubricating coatings presents a more pressing demand for improving performance. Herein, octa-amino polyhedral oligomeric silsesquioxane (POSS) were covalently grafted onto polyimide (PI) matrix. The effect of POSS on the mechanical properties of the PI-based composite coatings and the tribological properties of PI/PTFE based lubricating coatings before and after modification were investigated. As expected, compared with the pure PI, the POSS-PI nano-materials exhibited 31.6% and 32.7% enhancements in tensile strength and nano-hardness without discernable decrease in breaking elongation. Additionally, the wear rate significantly decreased by 54.9% with the addition of OPOSS. The enhancement of wear resistance could be attributed to the improved cohesion strength and load-bearing capacity of the PI/PTFE composite coating reinforced by POSS.
引用
收藏
页数:13
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共 43 条
[1]   Atomic-Oxygen-Durable and Electrically-Conductive CNT-POSS-Polyimide Flexible Films for Space Applications [J].
Atar, Nurit ;
Grossman, Eitan ;
Gouzman, Irina ;
Bolker, Asaf ;
Murray, Vanessa J. ;
Marshall, Brooks C. ;
Qian, Min ;
Minton, Timothy K. ;
Hanein, Yael .
ACS APPLIED MATERIALS & INTERFACES, 2015, 7 (22) :12047-12056
[2]   Synthesis and characterization of polyhedral oligomeric silsesquioxane-siloxane-modified polyimide hybrid nanocomposites [J].
Chandramohan, A. ;
Nagendiran, S. ;
Alagar, M. .
JOURNAL OF COMPOSITE MATERIALS, 2012, 46 (07) :773-781
[3]   Mechano-adaptive thin film of graphene-based polymeric nanocomposite for enhancement of lubrication properties [J].
Chouhan, Ajay ;
Sarkar, Tarun K. ;
Kumari, Sangita ;
Sivakumar, K. L. N. ;
Sugimura, H. ;
Khatri, Om P. .
APPLIED SURFACE SCIENCE, 2021, 538
[4]   Recent Developments in the Chemistry of Cubic Polyhedral Oligosilsesquioxanes [J].
Cordes, David B. ;
Lickiss, Paul D. ;
Rataboul, Franck .
CHEMICAL REVIEWS, 2010, 110 (04) :2081-2173
[5]   Hybrid Silicon-Based Organic/Inorganic Block Copolymers with Sol-Gel Active Moieties: Synthetic Advances, Self-Assembly and Applications in Biomedicine and Materials Science [J].
Czarnecki, Sebastian ;
Bertin, Annabelle .
CHEMISTRY-A EUROPEAN JOURNAL, 2018, 24 (14) :3354-3373
[6]   The significance of tribochemistry on the performance of PTFE-based coatings in CO2 refrigerant environment [J].
Dascalescu, D. ;
Polychronopoulou, K. ;
Polycarpou, A. A. .
SURFACE & COATINGS TECHNOLOGY, 2009, 204 (03) :319-329
[7]   Investigation of surface properties and mechanical and tribological behaviors of polyimide based composite coatings [J].
Demian, Camelia ;
Liao, Hanlin ;
Lachat, Remy ;
Costil, Sophie .
SURFACE & COATINGS TECHNOLOGY, 2013, 235 :603-610
[8]   Studies on thermal and dielectric properties of ether linked cyclohexyl diamine (ELCD)-based polyimide POSS nanocomposites (POSS-PI) [J].
Devaraju, S. ;
Vengatesan, M. R. ;
Alagar, M. .
HIGH PERFORMANCE POLYMERS, 2011, 23 (02) :99-111
[9]   Rheological and Tribological Properties of Carbon Nanotube/Thermoplastic Nanocomposites Incorporating Inorganic Fullerene-Like WS2 Nanoparticles [J].
Diez-Pascual, Ana M. ;
Naffakh, Mohammed ;
Marco, Carlos ;
Ellis, Gary .
JOURNAL OF PHYSICAL CHEMISTRY B, 2012, 116 (27) :7959-7969
[10]   Surfactant assisted and in situ formed micro liquid metal as excellent lubricant additive in polyimide coating [J].
Dong, Lisong ;
Wu, Jian ;
Cao, Danyang ;
Feng, Xin ;
Zhu, Jiahua ;
Lu, Xiaohua ;
Mu, Liwen .
TRIBOLOGY INTERNATIONAL, 2021, 159