Electrospun nanofibrous adsorbents for uranium extraction from seawater

被引:122
作者
Xie, Siyuan [1 ,2 ]
Liu, Xiyan [1 ]
Zhang, Bowu [1 ]
Ma, Hongjuan [1 ]
Ling, Changjian [1 ]
Yu, Ming [1 ]
Li, Linfan [1 ]
Li, Jingye [1 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Appl Phys, CAS Ctr Excellence TMSR Energy Syst, Shanghai 201800, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
基金
中国国家自然科学基金;
关键词
HIGHLY EFFICIENT; MERCURY POROSIMETRY; POLYMERIC ADSORBENT; CARBON NANOTUBES; AMIDOXIME; ADSORPTION; RECOVERY; URANYL; FIBER; SORPTION;
D O I
10.1039/c4ta06120a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Here we report a nanoadsorbent design, which integrates the high affinity of amidoxime (AO) groups and size effect of nanomaterials in nanofibrous composite mats prepared by a two-nozzle electrospinning process, for the adsorption of uraniumin simulated seawater with an uptake capacity of 1.6 mg U g(-1) adsorbent in the presence of massive amounts of interference ions.
引用
收藏
页码:2552 / 2558
页数:7
相关论文
共 61 条
[1]   Tuning Amidoximate to Enhance Uranyl Binding: A Density Functional Theory Study [J].
Abney, Carter W. ;
Liu, Shubin ;
Lin, Wenbin .
JOURNAL OF PHYSICAL CHEMISTRY A, 2013, 117 (45) :11558-11565
[2]   Functional materials by electrospinning of polymers [J].
Agarwal, Seema ;
Greiner, Andreas ;
Wendorff, Joachim H. .
PROGRESS IN POLYMER SCIENCE, 2013, 38 (06) :963-991
[3]   A Review: Studies on Uranium Removal Using Different Techniques. Overview [J].
Aly, Mohsen M. ;
Hamza, Mohammed F. .
JOURNAL OF DISPERSION SCIENCE AND TECHNOLOGY, 2013, 34 (02) :182-213
[4]  
[Anonymous], RECENT INT R D ACTIV
[5]  
[Anonymous], 2014, UR 2014 RES PROD DEM
[6]   Surface modification of ionic liquid-spun chitin fibers for the extraction of uranium from seawater: seeking the strength of chitin and the chemical functionality of chitosan [J].
Barber, Patrick S. ;
Kelley, Steven P. ;
Griggs, Chris S. ;
Wallace, Sergei ;
Rogers, Robin D. .
GREEN CHEMISTRY, 2014, 16 (04) :1828-1836
[7]   Highly selective extraction of the uranyl ion with hydrophobic amidoxime-functionalized ionic liquids via η2 coordination [J].
Barber, Patrick S. ;
Kelley, Steven P. ;
Rogers, Robin D. .
RSC ADVANCES, 2012, 2 (22) :8526-8530
[8]   Highly porous and stable metal-organic frameworks for uranium extraction [J].
Carboni, Michael ;
Abney, Carter W. ;
Liu, Shubin ;
Lin, Wenbin .
CHEMICAL SCIENCE, 2013, 4 (06) :2396-2402
[9]   Electrospinning: designed architectures for energy conversion and storage devices [J].
Cavaliere, Sara ;
Subianto, Surya ;
Savych, Iuliia ;
Jones, Deborah J. ;
Roziere, Jacques .
ENERGY & ENVIRONMENTAL SCIENCE, 2011, 4 (12) :4761-4785
[10]   Electrospinning of Calixarene-Functionalized Polyacrylonitrile Nanofiber Membranes and Application as an Adsorbent and Catalyst Support [J].
Chen, Ming ;
Wang, Chengjiao ;
Fang, Wei ;
Wang, Jing ;
Zhang, Wang ;
Jin, Gong ;
Diao, Guowang .
LANGMUIR, 2013, 29 (38) :11858-11867