Membrane pilot plant trials of CO2 separation from flue gas

被引:37
作者
Scholes, Colin A. [1 ]
Qader, Abdul [2 ]
Stevens, Geoff W. [3 ]
Kentish, Sandra E. [1 ]
机构
[1] Univ Melbourne, Dept Chem & Biomol Engn, Melbourne, Vic 3010, Australia
[2] Univ Melbourne, Melbourne, Vic 3010, Australia
[3] Univ Melbourne, Dept Chem & Biomol Engn, Chem Engn, Melbourne, Vic 3010, Australia
关键词
membrane; carbon dioxide; flue gas; pilot plant; facilitated transport; CARBON-DIOXIDE CAPTURE; SPIRAL WOUND MODULES; WATER-VAPOR; FACILITATED TRANSPORT; POLYMERIC MEMBRANES; POLYIMIDE MEMBRANES; MASS-TRANSFER; FLOW; PERMEATION; CHANNELS;
D O I
10.1002/ghg.1498
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Industrial trials of membrane separation of CO2 from flue gas generated by a lignite-fired power station are reported. A hollow fiber Air Products PRISM and a spiral wound Dow Filmtec (R) NF3838/30FF membrane were separately trialed. The CO2 permeance and selectivity through the PRISM membrane fell significantly in the initial hours of operation, reflecting competitive sorption effects and concentration polarisation. Alternatively, the wet flue gas enabled a facilitated transport mechanism to operate for the NF3838/30FF membrane and the CO2 permeance and selectivity increased significantly compared to the dry membrane. Standard correlations were able to simulate the pressure drops through the modules.(c) 2015 Society of Chemical Industry and John Wiley & Sons, Ltd
引用
收藏
页码:229 / 237
页数:9
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