Defect MoS2 and Ti3C2 nanosheets co-assisted CdS to enhance visible-light driven photocatalytic hydrogen production

被引:23
作者
Wang, Yingrui [1 ,2 ]
Liu, Chao [1 ]
Kong, Cui [1 ]
Zhang, Fengjun [1 ,3 ]
机构
[1] Anhui Jianzhu Univ, Key Lab Funct Mol Design & Interface Proc, Hefei 230601, Anhui, Peoples R China
[2] Anhui Jianzhu Univ, Construct Econ & Real Estate Management Res Ctr, Hefei 230601, Anhui, Peoples R China
[3] Anhui Jianzhu Univ, Anhui Key Lab Adv Bldg Mat, Hefei 230022, Anhui, Peoples R China
关键词
Mo vacancy; Defect MoS2/Ti3C2/CdS; Photocatalytic hydrogen production; HETEROGENEOUS HYBRID; EFFICIENT COCATALYST; H-2; EVOLUTION; NANORODS; HETEROSTRUCTURE; PERFORMANCE; COMPOSITES; SEPARATION; SITES; MXENE;
D O I
10.1016/j.colsurfa.2022.129746
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The addition of a co-catalyst is one of the most effective ways to enhance the performance of CdS photocatalytic hydrogen production. In this work, ternary photocatalysts with Defect MoS2 and Ti3C2 acting synergistically on CdS are explored. The experimental results showed that the Defect MoS2/Ti3C2/CdS photocatalyst had excellent photocatalytic hydrogen production performance of 14.1 mmol h(-1)g(-1), which was 18.5, 12.4, and 1.2 times higher than that of CdS, Ti3C2/CdS and Defect MoS2/CdS, respectively. Defect MoS2 and Ti3C2 synergistically interact with CdS and form heterojunctions, which improve the carrier separation efficiency and effectively suppress the recombination of photogenerated carriers. A possible photocatalytic hydrogen production mecha-nism of Defect MoS2/Ti3C2/CdS is also proposed. The dual co-catalysts of Defect MoS2 and Ti3C2 demonstrated in this paper provide a feasible approach for the development of composite catalysts.
引用
收藏
页数:9
相关论文
共 50 条
  • [31] High-performance visible-light-driven MoS2/CdZnS nanorods for photocatalytic hydrogen production by water splitting
    Fu, Haitao
    Zhao, Hongming
    Li, Xiaolang
    Chen, Fu
    Yang, Xiaohong
    Xiong, Shixian
    Li, Song
    An, Xizhong
    [J]. POWDER TECHNOLOGY, 2023, 429
  • [32] Facile preparation of BiOCl/Ti3C2 hybrid photocatalyst with enhanced visible-light photocatalytic activity
    Lian, Weiwei
    Wang, Libo
    Wang, Xiaolong
    Shen, Changjie
    Zhou, Aiguo
    Hu, Qianku
    [J]. FUNCTIONAL MATERIALS LETTERS, 2019, 12 (01)
  • [33] OD/2D nanocomposite visible light photocatalyst for highly stable and efficient hydrogen generation via recrystallization of CdS on MoS2 nanosheets
    Ma, Fukun
    Wu, Yongzhong
    Shao, Yongliang
    Zhong, Yueyao
    Lv, Jiaxin
    Hao, Xiaopeng
    [J]. NANO ENERGY, 2016, 27 : 466 - 474
  • [34] Effective orientation control of photogenerated carrier separation via rational design of a Ti3C2(TiO2)@CdS/MoS2 photocatalytic system
    Ai, Zizheng
    Shao, Yongliang
    Chang, Bin
    Huang, Baibiao
    Wu, Yongzhong
    Hao, Xiaopeng
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 242 : 202 - 208
  • [35] The heterojunction between 3D ordered macroporous TiO2 and MoS2 nanosheets for enhancing visible-light driven CO2 reduction
    Li, Yifei
    Tang, Junjie
    Wei, Yuechang
    He, Wenjie
    Tang, Zhiling
    Zhang, Xiao
    Xiong, Jing
    Zhao, Zhen
    [J]. JOURNAL OF CO2 UTILIZATION, 2021, 51
  • [36] Facile ultrasound-driven formation and deposition of few-layered MoS2 nanosheets on CdS for highly enhanced photocatalytic hydrogen evolution
    Qian, Xianhao
    Zhang, Jingyi
    Guo, Zhuang
    Liu, Shuzi
    Liu, Jinxin
    Lin, Jun
    [J]. APPLIED SURFACE SCIENCE, 2019, 481 : 795 - 801
  • [37] Two dimensional mixed heterostructure of Ti3C2/MoS2 for improving photoelectric response
    Xu, Xiang
    Lu, Chunhui
    Zhang, Ying
    Bai, Xing
    Liu, Zenghui
    Xu, Xinlong
    Hua, Dengxin
    [J]. APPLIED PHYSICS EXPRESS, 2021, 14 (10)
  • [38] MoS2/CdS rod-like nanocomposites as high-performance visible light photocatalyst for water splitting photocatalytic hydrogen production
    Zhao, Hongming
    Fu, Haitao
    Yang, Xiaohong
    Xiong, Shixian
    Han, Dezhi
    An, Xizhong
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (13) : 8247 - 8260
  • [39] Latest progress in photocatalytic hydrogen production using MXene (Ti3C2)/MOFs 3 C 2 )/MOFs composite: A review
    Fattah-alhosseini, Arash
    Sangarimotlagh, Zahra
    Karbasi, Minoo
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2024, 79 : 771 - 790
  • [40] Grinding-assisted heterogeneous nucleation of BiOAc on MoS2 nanoflowers to heterojunction with good visible-light photocatalytic performance
    Liu, Huanzhen
    Han, Qiaofeng
    Jia, Xuemei
    Shen, Zichen
    [J]. PARTICUOLOGY, 2021, 56 : 132 - 141