New Strategy To Enhance CO2 Capture over a Nanoporous Polyethylenimine Sorbent

被引：20
|
作者：
Wang, Xiaoxing [1 ]
Song, Chunshan [1 ,2 ]
机构：
[1] Penn State Univ, Clean Fuels & Catalysis Program, EMS Energy Inst, Dept Energy & Mineral Engn, 209 Acad Projects Bldg, University Pk, PA 16802 USA
[2] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA
来源：
ENERGY & FUELS | 2014年 / 28卷 / 12期
关键词：
MESOPOROUS-MOLECULAR-SIEVE; CARBON-DIOXIDE CAPTURE; SOLID AMINE SORBENTS; FLUE-GAS; BASKET SORBENTS; POROUS SILICA; HIGH-CAPACITY; ADSORPTION; ADSORBENT; REMOVAL;
D O I：
10.1021/ef501997q
中图分类号：
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号：
0807 ; 0820 ;
摘要：
A study was conducted to propose a new strategy to enhance CO2 capture over a nanoporous polyethylenimine sorbent. It was demonstrated that only 1 mol of amine sites was needed to sorb 1 mol of CO2 in the presence of K2CO3. It was observed that as a result of this, the amine efficiency could be doubled theoretically and CO2 capture capacity could be enhanced. Sorbents developed in this cost-effective method provided great potential to capture CO2 more efficiently and had a major impact on the advancement of current CCUS technologies. Fumed silica was used as a support to demonstrate the success of the proposed strategy for CO2 capture enhancement.
引用
收藏
页码：7742 / 7745
页数：4
相关论文
共 50 条
  • [1] Polyethylenimine-Magadiite Layered Silicate Sorbent for CO2 Capture
    Vieira, Romulo B.
    Pastore, Heloise O.
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (04) : 2472 - 2480
  • [2] Development of silica-gel-supported polyethylenimine sorbent for CO2 capture
    Zhang, Zhonghua
    Ma, Xiaoliang
    Song, Chunshan
    Wang, Yonggang
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2010, 240
  • [3] Polyethylenimine loaded nanoporous carbon with ultra-large pore volume for CO2 capture
    Tang, Zhihong
    Han, Zhuo
    Yang, Guangzhi
    Yang, Junhe
    APPLIED SURFACE SCIENCE, 2013, 277 : 47 - 52
  • [4] CO2 capture from the atmosphere using nanoporous-material-supported polyethylenimine sorbents
    Ma, Xiaoliang
    Zhang, Zhonghua
    Zhu, Jian
    Wang, Xiaoxing
    Song, Chunshan
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2011, 241
  • [5] Development of a new clay supported polyethylenimine composite for CO2 capture
    Wang, Weilong
    Xiao, Jing
    Wei, Xiaolan
    Ding, Jing
    Wang, Xiaoxing
    Song, Chunshan
    APPLIED ENERGY, 2014, 113 : 334 - 341
  • [6] Steam Regeneration of Polyethylenimine-Impregnated Silica Sorbent for Postcombustion CO2 Capture: A Multicyclic Study
    Sandhu, Navjot Kaur
    Pudasainee, Deepak
    Sarkar, Partha
    Gupta, Rajender
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2016, 55 (07) : 2210 - 2220
  • [7] The Nanofibrous CaO Sorbent for CO2 Capture
    Rodaev, Vyacheslav V.
    Razlivalova, Svetlana S.
    Tyurin, Alexander, I
    Vasyukov, Vladimir M.
    NANOMATERIALS, 2022, 12 (10)
  • [8] CO2 capture over molecular basket sorbent: Sorption mechanism study
    Wang, Xiaoxing
    Ma, Xiaoliang
    Schwartz, Viviane
    Clark, Jason C.
    Overbury, Steven H.
    Xu, Xiaochun
    Song, Chunshan
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2011, 242
  • [9] New porous MgO sorbent to capture CO2 at 473 K
    Li, Yan Yan
    Wan, Mi Mi
    Lin, Wei Gang
    Wang, Ying
    Zhu, Jian Hua
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2014, 248
  • [10] Polyethylenimine-Magadiite Layered Silicate Sorbent for CO2 Capture (vol 48, pg 2472, 2014)
    Vieira, Romulo B.
    Pastore, Heloise O.
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2016, 50 (23) : 13173 - 13173
12345