A Non-interpenetrated Microporous Bi-pillared-Layer Framework: Synthesis, Structure and Photoluminescence Properties

被引：0
|
作者：
Lu, Jitao [1 ]
Sui, Haiyan [1 ]
Meng, Dandan [1 ]
Meng, Qingguo [1 ]
机构：
[1] Weifang Univ, Coll Chem Engn & Environm Chem, Weifang 261061, Peoples R China
来源：
JOURNAL OF INORGANIC AND ORGANOMETALLIC POLYMERS AND MATERIALS | 2015年 / 25卷 / 04期
关键词：
5-Hydroxyisophthalic acid; Microporous; Bi-pillared-layer; MOFs; Photoluminescence; METAL-ORGANIC FRAMEWORK; COORDINATION POLYMERS; CRYSTAL-STRUCTURES; GAS-SORPTION; ANTITUMOR-ACTIVITY; HYDROGEN STORAGE; LIGAND; DESIGN; ADSORPTION; COMPLEXES;
D O I：
10.1007/s10904-015-0194-5
中图分类号：
O63 [高分子化学（高聚物）];
学科分类号：
070305 ; 080501 ; 081704 ;
摘要：
A non-interpenetrated microporous bi-pillared-layer framework of Zn(II), {[Zn(hip)(4,4'-bipy)](DMA)center dot(4H(2)O)}(n) (1) (H(2)hip = 5-hydroxyisophthalic acid; 4,4'-bipy = 4,4'-bipyridine; DMA = N,N'-diethylformamide) composed of mixed ligand system has been synthesized and structurally characterized. The hip linkers form a 2D corrugated sheet of {Zn(hip)}(n) by linking the secondary building unit of Zn-2(CO2)(2) in the bc plane, which are further connected by double 4,4'-bipy pillars resulting in a bi-pillared-layer type 3D framework. The 3D framework is non-interpenetrated and exhibits a 3D channel structure occupied by the guest DMA molecules. The thermal stability and luminescent properties were also investigated.
引用
收藏
页码：936 / 941
页数：6
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