Novel coordination polymers with 1,4-di(benzimidazole-1-yl)benzene modulated by an anion: Syntheses, structures and properties

被引：4

作者：

Li Lei ^{[1
]}

Hu TongLiang ^{[1
]}

Zeng YongFei ^{[1
]}

Bu XianHe ^{[1
]}

机构：

[1] Nankai Univ, Dept Chem, TKL Met & Mol Based Mat Chem, Tianjin 300071, Peoples R China

来源：

SCIENCE CHINA-CHEMISTRY | 2010年 / 53卷 / 10期

基金：

中国国家自然科学基金;

关键词：

anion effect; coordination polymer; fluorescence; magnetic properties; structure; METAL-ORGANIC FRAMEWORKS; SECONDARY BUILDING UNITS; N-ARYLATION; LIGANDS; COMPLEXES; MOLECULES; EFFICIENT; CHANNELS; NETWORK; PHOTOLUMINESCENCE;

D O I：

10.1007/s11426-010-4101-1

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Three novel coordination polymers, {[Co(L)(SO4)(H2O)](CH3OH)}(infinity) (1), {[Cd(L)(2)(SiF6)](H2O)}(infinity) (2) and [Zn(L)(NO3)(2)](infinity) (3), synthesized from 1,4-di(benzimidazole-1-yl)benzene (L), have been characterized by infrared spectroscopy, elemental analysis and single crystal X-ray diffraction. Compounds 1-3 exhibit different structures. Complex 1 has a 3-D diamond network containing 1-D Co-II chains connected by SO42- anions; 2 has a 3-D alpha-Po framework with 1-D porous channels along the c axis; and 3 has a 1-D zig-zag chain structure with a 2-D supramolecular network based on pi-pi interactions. The magnetic properties of 1 and the solid state fluorescence spectra of 2 and 3 have also been explored.

引用

页码：2170 / 2176

页数：7

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