2D Salphen-based heteropore covalent organic frameworks for highly efficient electrocatalytic water oxidation

被引：19

作者：

Wang, Lin-Lin ^{[1
]}

Zhang, Wen-Da ^{[1
]}

Li, Tao ^{[1
]}

Yan, Xiaodong ^{[1
]}

Gao, Jie ^{[1
]}

Chen, Yu-Xuan ^{[1
]}

Shi, Ya-Xiang ^{[1
]}

Gu, Zhi-Guo ^{[1
,2
]}

机构：

[1] Jiangnan Univ, Sch Chem & Mat Engn, Key Lab Synthet & Biol Colloids, Minist Educ, Wuxi 214122, Jiangsu, Peoples R China

[2] Jiangnan Univ, Int Joint Res Ctr Photorespons Mol & Mat, Sch Chem & Mat Engn, Wuxi 214122, Jiangsu, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2021年 / 57卷 / 97期

基金：

中国国家自然科学基金;

关键词：

NANOSHEETS; CRYSTALLINE; POLYMERS;

D O I：

10.1039/d1cc04369b

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The construction of heteroporous covalent organic frameworks (COFs) is still a challenge. Herein, a series of 2D COFs with hexagonal and quadrilateral pores were constructed via in situ salphen or metal salphen formation. Metallized salphen-based COFs can be used as electrocatalysts towards water oxidation with an overpotential of 266 mV at 10 mA cm(-2).

引用

页码：13162 / 13165

页数：4

共 37 条

[1] Sub-stoichiometric 2D covalent organic frameworks from tri- and tetratopic linkers [J].

Banerjee, Tanmay ;

Haase, Frederik ;

Trenker, Stefan ;

Biswal, Bishnu P. ;

Savasci, Goekcen ;

Duppel, Viola ;

Moudrakovski, Igor ;

Ochsenfeld, Christian ;

Lotsch, Bettina V. .

NATURE COMMUNICATIONS, 2019, 10 (1)

[2] Covalent Organic Frameworks: Chemical Approaches to Designer Structures and Built-In Functions [J].

Chen, Xinyi ;

Geng, Keyu ;

Liu, Ruoyang ;

Tan, Ke Tian ;

Gong, Yifan ;

Li, Zhongping ;

Tao, Shanshan ;

Jiang, Qiuhong ;

Jiang, Donglin .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2020, 59 (13) :5050-5091

[3] 3D Porous Crystalline Polyimide Covalent Organic Frameworks for Drug Delivery [J].

Fang, Qianrong ;

Wang, Junhua ;

Gu, Shuang ;

Kaspar, Robert B. ;

Zhuang, Zhongbin ;

Zheng, Jie ;

Guo, Hongxia ;

Qiu, Shilun ;

Yan, Yushan .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (26) :8352-8355

[4] Covalent Organic Frameworks: Design, Synthesis, and Functions [J].

Geng, Keyu ;

He, Ting ;

Liu, Ruoyang ;

Dalapati, Sasanka ;

Tan, Ke Tian ;

Li, Zhongping ;

Tao, Shanshan ;

Gong, Yifan ;

Jiang, Qiuhong ;

Jiang, Donglin .

CHEMICAL REVIEWS, 2020, 120 (16) :8814-8933

[5] Solving the COF trilemma: towards crystalline, stable and functional covalent organic frameworks [J].

Haase, Frederik ;

Lotsch, Bettina V. .

CHEMICAL SOCIETY REVIEWS, 2020, 49 (23) :8469-8500

[6] Chiral Covalent Organic Frameworks with High Chemical Stability for Heterogeneous Asymmetric Catalysis [J].

Han, Xing ;

Xia, Qingchun ;

Huang, Jinjing ;

Liu, Yan ;

Tan, Chunxia ;

Cui, Yong .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2017, 139 (25) :8693-8697

[7] Two-dimensional graphdiyne analogue Co-coordinated porphyrin covalent organic framework nanosheets as a stable electrocatalyst for the oxygen evolution reaction [J].

Huang, Hao ;

Li, Fumin ;

Zhang, Ying ;

Chen, Yu .

JOURNAL OF MATERIALS CHEMISTRY A, 2019, 7 (10) :5575-5582

[8] [6+6] Schiff-base macrocycles with 12 imines: giant analogues of cyclohexane [J].

Hui, Joseph K. -H. ;

MacLachlan, Mark J. .

CHEMICAL COMMUNICATIONS, 2006, (23) :2480-2482

[9] Covalent Organic Frameworks: An Amazing Chemistry Platform for Designing Polymers [J].

Jiang, Donglin .

CHEM, 2020, 6 (10) :2461-2483

[10] Directly anchoring 2D NiCo metal-organic frameworks on few-layer black phosphorus for advanced lithium-ion batteries [J].

Jin, Jun ;

Zheng, Yun ;

Huang, Shao-zhuan ;

Sun, Ping-ping ;

Srikanth, Narasimalu ;

Kong, Ling Bing ;

Yan, Qingyu ;

Zhou, Kun .

JOURNAL OF MATERIALS CHEMISTRY A, 2019, 7 (02) :783-790

← 1 2 3 4 →