Origin and distribution of polyaromatic hydrocarbons and polychlorobiphenyls in urban effluents to wastewater treatment plants of the Paris area (France)

被引:90
作者
Blanchard, M [1 ]
Teil, MJ [1 ]
Ollivon, D [1 ]
Garban, B [1 ]
Chestérikoff, C [1 ]
Chevreuil, M [1 ]
机构
[1] Univ Paris 06, Ecole Prat Hautes Etud UMR Sisyphe 7619, Lab Hydrol & Environm, F-75252 Paris 05, France
关键词
polychlorobiphenyl; polyaromatic hydrocarbon; wastewater treatment plant; sewage sludge;
D O I
10.1016/S0043-1354(01)00078-1
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Polyaromatic hydrocarbons (PAHs) and polychlorobiphenyls (PCBs), were investigated in urban effluents to wastewater treatment plants in the Paris area (France), under different meteorological conditions. The Acheres plant was considered with special attention because of its particular features. Wastewater PAH concentration level was 6 fold higher than that of PCBs. In March, PCB concentrations did not vary whatever the meteorological conditions whereas, for PAHs, they were markedly higher during rainy episodes. In September, concentrations of both pollutants increased due to rainy weather. The rise was 30 fold stronger for PAHs. Daily fluxes displayed the same trends. This suggests that the contribution of atmospheric wet deposition to wastewater contamination prevails for PCBs. In contrast, PAHs appeared to originate mainly from urban runoff processes. (C) 2001 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:3679 / 3687
页数:9
相关论文
共 27 条
[1]   TOXIC EQUIVALENCY FACTORS FOR DIOXIN-LIKE PCBS - REPORT ON A WHO-ECEH AND IPCS CONSULTATION, DECEMBER 1993 [J].
AHLBORG, UG ;
BECKING, GC ;
BIRNBAUM, LS ;
BROUWER, A ;
DERKS, HJGM ;
FEELEY, M ;
GOLOR, G ;
HANBERG, A ;
LARSEN, JC ;
LIEM, AKD ;
SAFE, SH ;
SCHLATTER, C ;
WAERN, F ;
YOUNES, M ;
YRJANHEIKKI, E .
CHEMOSPHERE, 1994, 28 (06) :1049-1067
[2]   Improvements to the UK PCDD/F and PCB atmospheric emission inventory following an emissions measurement programme [J].
Alcock, RE ;
Gemmill, R ;
Jones, KC .
CHEMOSPHERE, 1999, 38 (04) :759-770
[3]   Dioxin-like PCBs in the environment - Human exposure and the significance of sources [J].
Alcock, RE ;
Behnisch, PA ;
Jones, KC ;
Hagenmaier, H .
CHEMOSPHERE, 1998, 37 (08) :1457-1472
[4]   REDUCTIVE DECHLORINATION OF POLYCHLORINATED-BIPHENYLS IN ANAEROBIC SEDIMENTS [J].
ALDER, AC ;
HAGGBLOM, MM ;
OPPENHELMER, SR ;
YOUNG, LY .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1993, 27 (03) :530-538
[5]   PCB and PAH impacts on cytochrome P-450-dependent oxidases in roach (Rutilus rutilus) from the Seine River (France) [J].
Blanchard, M ;
Teil, AM ;
Carru, AM ;
Ollivon, D ;
Garban, B ;
Chesterikoff, A ;
Chevreuil, M .
ARCHIVES OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY, 1999, 37 (02) :242-250
[6]   Organochlorine distribution and mono-orthosubstituted PCB pattern in the roach (Rutilus rutilus) from the River Seine [J].
Blanchard, M ;
Teil, MJ ;
Carru, AM ;
Chesterikoff, A ;
Chevreuil, M .
WATER RESEARCH, 1997, 31 (06) :1455-1461
[7]   Comparison of polycyclic aromatic compounds and heavy metals contents in sewage sludges from industrialized and non-industrialized region [J].
Bodzek, D ;
Janoszka, B .
WATER AIR AND SOIL POLLUTION, 1999, 111 (1-4) :359-369
[8]   A street deposit sampling method for metal and hydrocarbon contamination assessment [J].
Bris, FJ ;
Garnaud, S ;
Apperry, N ;
Gonzalez, A ;
Mouchel, JM ;
Chebbo, G ;
Thévenot, DR .
SCIENCE OF THE TOTAL ENVIRONMENT, 1999, 235 (1-3) :211-220
[9]   Microbial dechlorination of polychlorinated biphenyls in anaerobic sewage sludge [J].
Chang, BV ;
Chou, SW ;
Yuan, SY .
CHEMOSPHERE, 1999, 39 (01) :45-54
[10]  
CHEVREUIL M, 1998, SEINE SON BASSIN FON, P439