Disalignment rate coefficient of neon excited atoms due to helium atom collisions at low temperatures

被引:10
作者
Seo, M
Shimamura, T
Furutani, T
Hasuo, M [1 ]
Bahrim, C
Fujimoto, T
机构
[1] Kyoto Univ, Grad Sch Engn, Dept Engn Phys & Mech, Kyoto 6068501, Japan
[2] Lamar Univ, Dept Chem & Phys, Beaumont, TX 77710 USA
关键词
D O I
10.1088/0953-4075/36/9/317
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Disalignment of neon excited atoms in the fine-structure 2p(i) levels (in Paschen notation) of the 2p(5)3p configuration is investigated in a helium-neon glow discharge at temperatures between 15 and 77 K;l At several temperatures, we plot the disalignment rate as a function of the helium atom density for Ne*(2p(2) or 2p(7)) + He(1s(2)) collisions. The slope of this dependence gives the disalignment rate coefficient. For both collisions, the experimental data for the disalignment rate coefficient show a more rapid decrease with the decrease in temperature below 40 K than our quantum close-coupling calculations based on the model potential of Hennecart and Masnou-Seeums (19, 851 Phys. B: At. Mol. Phys. 18 657). This finding suggests that the disalignment cross Section rapidly decreases below a few millielectronvolts, in disagreement with our theoretical quantum calculations which predict a. strong increase below 1 meV The disagreement suggests that the long-range electrostatic potentials are significantly more repulsive, than in the aforementioned model.
引用
收藏
页码:1885 / 1898
页数:14
相关论文
共 17 条
[1]   Longitudinal alignment transfer between fine-structure levels in Ne*(2p53p)+He collisions.: Comparison between cell experiments and quantum calculations [J].
Bahrim, C ;
Hennecart, D ;
Kucal, H ;
Masnou-Seeuws, F .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1999, 32 (13) :3091-3105
[2]   Absolute cross sections with polarization effects in Ne-*(2p(5)3p)+He collisions: A detailed comparison between theory and experiment [J].
Bahrim, C ;
Kucal, H ;
MasnouSeeuws, F .
PHYSICAL REVIEW A, 1997, 56 (02) :1305-1320
[3]   Quantal calculations for alignment relaxation in Ne*(2p(5)3p)+He collisions [J].
Bahrim, C ;
Kucal, H ;
Dulieu, O ;
MasnouSeeuws, F .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1997, 30 (22) :L797-L804
[4]   Long-range diatomic s+p potentials of heavy rare gases [J].
Doery, MR ;
Vredenbregt, EJD ;
Tempelaars, JGC ;
Beijerinck, HCW ;
Verhaar, BJ .
PHYSICAL REVIEW A, 1998, 57 (05) :3603-3620
[5]   Plasma polarization spectroscopy [J].
Fujimoto, T ;
Kazantsev, SA .
PLASMA PHYSICS AND CONTROLLED FUSION, 1997, 39 (09) :1267-1294
[6]   MODEL POTENTIAL CALCULATIONS FOR THE EXCITED-STATES OF NE-STAR-HE AND NE-STAR-NE - APPLICATION TO THE INTERPRETATION OF COLLISION EXPERIMENTS [J].
HENNECART, D ;
MASNOUSEEUWS, F .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1985, 18 (04) :657-689
[7]   Coupled-channel calculations of excited-atom collisions [J].
Hickman, AP .
INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY, 1997, 16 (02) :177-199
[8]   DISALIGNMENT OF EXCITED NEON ATOMS DUE TO ELECTRON AND ION COLLISIONS [J].
HIRABAYASHI, A ;
NAMBU, Y ;
HASUO, M ;
FUJIMOTO, T .
PHYSICAL REVIEW A, 1988, 37 (01) :83-88
[9]   COLLISION-INDUCED INTRAMULTIPLET MIXING FOR NE STAR-STAR ((2P)5(3P))+HE - EXPERIMENTS AND QUANTUM CALCULATIONS [J].
MANDERS, MPI ;
DRIESSEN, JPJ ;
BEIJERINCK, HCW ;
VERHAAR, BJ .
PHYSICAL REVIEW A, 1988, 37 (09) :3237-3253
[10]   MOLECULAR THEORY OF ATOMIC COLLISIONS - FINE-STRUCTURE TRANSITIONS [J].
MIES, FH .
PHYSICAL REVIEW A, 1973, 7 (03) :942-957