Determining the Effect of Plasma Pre-Treatment on Antimony Tin Oxide to Support Pt@Pd and the Oxygen Reduction Reaction Activity

被引:12
作者
Liu, Xiaoteng [1 ]
Zhang, Kui [1 ]
Lu, Jianwei [2 ]
Luo, Kun [3 ]
Gong, Jinlong [2 ]
Puthiyapura, Vinod K. [1 ]
Scott, Keith [1 ]
机构
[1] Newcastle Univ, Sch Chem Engn & Adv Mat, Merz Court, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England
[2] Tianjin Univ, Sch Chem Engn & Technol, Minist Educ, Key Lab Green Chem Technol, Tianjin 300072, Peoples R China
[3] Guilin Univ Technol, Coll Mat Sci & Engn, Minist Educ, Key Lab New Proc Technol Nonferrous Met & Mat, Guilin 541004, Peoples R China
基金
英国工程与自然科学研究理事会;
关键词
antimony tin oxide; durability; fuel cells; oxygen reduction reaction; plasma; FUEL-CELLS; GREENHOUSE GASES; CORE-SHELL; CATALYSTS; STABILITY; ELECTROCATALYSTS; HYDROCARBONS; CONVERSION; PLATINUM; PEMFCS;
D O I
10.1002/cctc.201500206
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This article reveals the effect of plasma pre-treatment on antimony tin oxide (ATO) nanoparticles. The effect is to allow Pt@Pd to be deposited homogeneously on the ATO surface with high dispersion and narrow particle size distribution. The Pt@Pd core-shell catalyst was prepared using the polyol method and shows a dramatic improvement towards ORR activity and durability.
引用
收藏
页码:1543 / 1546
页数:4
相关论文
共 21 条
[11]   Electrocatalytic corrosion of carbon support in PEMFC cathodes [J].
Roen, LM ;
Paik, CH ;
Jarvic, TD .
ELECTROCHEMICAL AND SOLID STATE LETTERS, 2004, 7 (01) :A19-A22
[12]   Enhanced electrocatalytic activity of CoTMPP-based catalysts for PEMFCs by plasma treatment [J].
Savastenko, N. A. ;
Brueser, V. ;
Brueser, M. ;
Anklam, K. ;
Kutschera, S. ;
Steffen, H. ;
Schmuhl, A. .
JOURNAL OF POWER SOURCES, 2007, 165 (01) :24-33
[13]   ELECTRICAL AND OPTICAL-PROPERTIES OF UNDOPED AND ANTIMONY-DOPED TIN OXIDE-FILMS [J].
SHANTHI, E ;
DUTTA, V ;
BANERJEE, A ;
CHOPRA, KL .
JOURNAL OF APPLIED PHYSICS, 1980, 51 (12) :6243-6251
[14]   Understanding and approaches for the durability issues of Pt-based catalysts for PEM fuel cell [J].
Shao, Yuyan ;
Yin, Geping ;
Gao, Yunzhi .
JOURNAL OF POWER SOURCES, 2007, 171 (02) :558-566
[15]   Ex situ and in situ stability studies of PEMFC catalysts [J].
Stevens, DA ;
Hicks, MT ;
Haugen, GM ;
Dahn, JR .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2005, 152 (12) :A2309-A2315
[16]   Characterization and stability of doped SnO2 anodes [J].
Vicent, F ;
Morallon, E ;
Quijada, C ;
Vazquez, JL ;
Aldaz, A ;
Cases, F .
JOURNAL OF APPLIED ELECTROCHEMISTRY, 1998, 28 (06) :607-612
[17]   SURFACE-AREA LOSS OF SUPPORTED PLATINUM IN POLYMER ELECTROLYTE FUEL-CELLS [J].
WILSON, MS ;
GARZON, FH ;
SICKAFUS, KE ;
GOTTESFELD, S .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1993, 140 (10) :2872-2877
[18]  
Yu EH, 2012, RSC ENERGY ENVIRON S, P227, DOI 10.1039/9781849734783-00227
[19]   Core-shell Pt modified Pd/C as an active and durable electrocatalyst for the oxygen reduction reaction in PEMFCs [J].
Zhang, Geng ;
Shao, Zhi-Gang ;
Lu, Wangting ;
Xie, Feng ;
Xiao, Hui ;
Qin, Xiaoping ;
Yi, Baolian .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2013, 132 :183-194
[20]   Direct conversion of greenhouse gases to synthesis gas and C4 hydrocarbons over zeolite HY promoted by a dielectric-barrier discharge [J].
Zhang, K ;
Eliasson, B ;
Kogelschatz, U .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2002, 41 (06) :1462-1468