Characterization and Elemental Composition of Atmospheric Aerosol Loads during Springtime Dust Storm in Western Saudi Arabia

被引:78
作者
Alghamdi, Mansour A. [1 ]
Almazroui, Mansour [2 ]
Shamy, Magdy [1 ]
Ana Redal, Maria [3 ]
Alkhalaf, Abdulrahman K. [2 ]
Hussein, Mahmoud A.
Khoder, Mamdouh I. [1 ,4 ]
机构
[1] King Abdulaziz Univ, Fac Meteorol Environm & Arid Land Agr, Dept Environm Sci, Jeddah 21413, Saudi Arabia
[2] King Abdulaziz Univ, Ctr Excellence Climate Change Res, Dept Meteorol, Jeddah 21413, Saudi Arabia
[3] Escuela Med Hosp Italiano Buenos Aires, Inst Ciencias Basicas & Med Expt, Unidad Med Mol Genom, Buenos Aires, DF, Argentina
[4] King Abdulaziz Univ, Ctr Excellence Environm Studies, Jeddah 21589, Saudi Arabia
关键词
PM10/PM2.5/PM1.0; Diurnal variation; Elemental composition; Dust storm; Jeddah; PARTICULATE AIR-POLLUTION; LONG-RANGE TRANSPORT; ASIAN DUST; SOURCE APPORTIONMENT; CHEMICAL-PROPERTIES; SEASONAL-VARIATIONS; PM2.5; CHINA; PM10; SEA;
D O I
10.4209/aaqr.2014.06.0110
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Dust storm is a common phenomenonand, a severe environmental hazard in western Saudi Arabia. In this study, simultaneous measurement of PM10, PM2.5 and PM1.0 and elemental compositions analysis of PM2.5 in Jeddah city during springtime (March 2012) dust storm (DS) and non-dust storm (non-DS) periods were carried out to investigate the impact of DS on the levels, characterization and elemental compositions of atmospheric particles. Results indicate that PM fractions concentrations were higher in DS environment compared to non-DS. The diurnal variation of PM fractions concentrations was uni-modal in non-DS environment and bimodal in DS. PM1.0/PM10, PM2.5/PM10 and PM2.5/PM2.5-10 ratios were relatively lower in DS, indicating that sand-dust events in spring carry much more coarse than fine particles to Jeddah. PM10, PM2.5 and PM1.0 in DS and PM10 and PM2.5 in non-DS might originate from similar sources. PM10, PM2.5, PM1.0 in DS and PM10 in non-DS were correlated negatively with relative humidity and positively with wind speed. PM2.5 and PM1.0 in non-DS were correlated positively with relative humidity and negatively with wind speed. The crustal elements accounted for 44.62 and 67.53% of the total concentrations of elements in non-DS and DS, respectively. The elements concentrations increased in DS, with highest DS/non-DS ratios for Ca, Si, Al and Fe. This indicates that the soil originating species contributed mainly in DS particles. The enrichment factors values and non-crustal fractions in both non-DS and DS indicate that the main sources of Na, Mg, Si, K, Ca, Ti, Cr, Mn, Fe, Rb and Sr are of a crustal type, whereas S, Cl, Co, Cu, Zn, Ga, As, Pb and Cd are anthropogenic. V and Ni in DS only are emitted from anthropogenic sources. The enrichment factors of these anthropogenic elements were lower in DS. They might originate mainly from local sources in Jeddah.
引用
收藏
页码:440 / U101
页数:20
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