Electrostatically Induced Superconductivity at the Surface of WS2

被引:143
作者
Jo, Sanghyun [1 ,2 ]
Costanzo, Davide [1 ,2 ]
Berger, Helmuth [3 ]
Morpurgo, Alberto F. [1 ,2 ]
机构
[1] Univ Geneva, DQMP, CH-1211 Geneva, Switzerland
[2] Univ Geneva, GAP, CH-1211 Geneva, Switzerland
[3] Ecole Polytech Fed Lausanne, Inst Phys Mat Complexe, CH-1015 Lausanne, Switzerland
基金
瑞士国家科学基金会;
关键词
WS2; transition metal dichalcogenides; ionic liquid gating; superconductivity; potential fluctuation; BKT transition; TRANSPORT-PROPERTIES; VALLEY POLARIZATION; MONOLAYER; MOS2; TRANSITION; CHEMISTRY; MOBILITY; DIODES; SPIN;
D O I
10.1021/nl504314c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We investigate transport through ionic liquid gated field effect transistors (FETs) based on exfoliated crystals of semiconducting WS2. Upon electron accumulation, at surface densities close to, or just larger than, 10(14) cm(2), transport exhibits metallic behavior with the surface resistivity decreasing pronouncedly upon cooling. A detailed characterization as a function of temperature and magnetic field clearly shows the occurrence of a gate-induced superconducting transition below a critical temperature Tc 4 K, a finding that represents the first demonstration of superconductivity in tungsten-based semiconducting transition metal dichalcogenides. We investigate the nature of superconductivity and find significant inhomogeneity, originating from the local detaching of the frozen ionic liquid from the WS2 surface. Despite the inhomogeneity, we find that in all cases where a fully developed zero resistance state is observed, different properties of the devices exhibit a behavior characteristic of a BerezinskiiKosterlitzThouless transition, as it could be expected in view of the two-dimensional nature of the electrostatically accumulated electron system
引用
收藏
页码:1197 / 1202
页数:6
相关论文
共 44 条
  • [1] Baugher BWH, 2014, NAT NANOTECHNOL, V9, P262, DOI [10.1038/NNANO.2014.25, 10.1038/nnano.2014.25]
  • [2] Intrinsic Electronic Transport Properties of High-Quality Monolayer and Bilayer MoS2
    Baugher, Britton W. H.
    Churchill, Hugh O. H.
    Yang, Yafang
    Jarillo-Herrero, Pablo
    [J]. NANO LETTERS, 2013, 13 (09) : 4212 - 4216
  • [3] POSSIBILITY OF VORTEX-ANTIVORTEX PAIR DISSOCIATION IN 2-DIMENSIONAL SUPERCONDUCTORS
    BEASLEY, MR
    MOOIJ, JE
    ORLANDO, TP
    [J]. PHYSICAL REVIEW LETTERS, 1979, 42 (17) : 1165 - 1168
  • [4] Broadening of the Berezinskii-Kosterlitz-Thouless superconducting transition by inhomogeneity and finite-size effects
    Benfatto, L.
    Castellani, C.
    Giamarchi, T.
    [J]. PHYSICAL REVIEW B, 2009, 80 (21)
  • [5] BEREZINSKII VL, 1972, SOV PHYS JETP-USSR, V34, P610
  • [6] Quantitative Determination of the Band Gap of WS2 with Ambipolar Ionic Liquid-Gated Transistors
    Braga, Daniele
    Lezama, Ignacio Gutierrez
    Berger, Helmuth
    Morpurgo, Alberto F.
    [J]. NANO LETTERS, 2012, 12 (10) : 5218 - 5223
  • [7] Valley-selective circular dichroism of monolayer molybdenum disulphide
    Cao, Ting
    Wang, Gang
    Han, Wenpeng
    Ye, Huiqi
    Zhu, Chuanrui
    Shi, Junren
    Niu, Qian
    Tan, Pingheng
    Wang, Enge
    Liu, Baoli
    Feng, Ji
    [J]. NATURE COMMUNICATIONS, 2012, 3
  • [8] Chhowalla M, 2013, NAT CHEM, V5, P263, DOI [10.1038/NCHEM.1589, 10.1038/nchem.1589]
  • [9] TOPOLOGICAL EXCITATIONS IN 2-DIMENSIONAL SUPERCONDUCTORS
    DONIACH, S
    HUBERMAN, BA
    [J]. PHYSICAL REVIEW LETTERS, 1979, 42 (17) : 1169 - 1172
  • [10] Gutierrez Lezama I., 2014, 23 MAT, P1