Unveiling the complex pattern of intermolecular interactions responsible for the stability of the DNA duplex

被引:20
作者
Altun, Ahmet [1 ]
Garcia-Rates, Miquel [1 ]
Neese, Frank [1 ]
Bistoni, Giovanni [1 ]
机构
[1] Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, Germany
关键词
ENERGY DECOMPOSITION ANALYSIS; GAUSSIAN-BASIS SETS; CORRELATED MOLECULAR CALCULATIONS; QUANTUM-CHEMICAL CALCULATIONS; DENSITY-FUNCTIONAL THEORY; SUGAR-PHOSPHATE BACKBONE; AUXILIARY BASIS-SETS; HARTREE-FOCK METHOD; BASE-PAIRS; NONCOVALENT INTERACTIONS;
D O I
10.1039/d1sc03868k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Herein, we provide new insights into the intermolecular interactions responsible for the intrinsic stability of the duplex structure of a large portion of human B-DNA by using advanced quantum mechanical methods. Our results indicate that (i) the effect of non-neighboring bases on the inter-strand interaction is negligibly small, (ii) London dispersion effects are essential for the stability of the duplex structure, (iii) the largest contribution to the stability of the duplex structure is the Watson-Crick base pairing - consistent with previous computational investigations, (iv) the effect of stacking between adjacent bases is relatively small but still essential for the duplex structure stability and (v) there are no cooperativity effects between intra-strand stacking and inter-strand base pairing interactions. These results are consistent with atomic force microscope measurements and provide the first theoretical validation of nearest neighbor approaches for predicting thermodynamic data of arbitrary DNA sequences.
引用
收藏
页码:12785 / 12793
页数:9
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