Time-Resolved Holography with Photoelectrons

被引:517
作者
Huismans, Y. [1 ]
Rouzee, A. [1 ,2 ]
Gijsbertsen, A. [1 ]
Jungmann, J. H. [1 ]
Smolkowska, A. S. [1 ]
Logman, P. S. W. M. [1 ]
Lepine, F. [3 ]
Cauchy, C. [3 ]
Zamith, S. [4 ,5 ]
Marchenko, T. [6 ]
Bakker, J. M. [7 ]
Berden, G. [7 ]
Redlich, B. [7 ]
van der Meer, A. F. G. [7 ]
Muller, H. G. [1 ]
Vermin, W. [8 ]
Schafer, K. J. [9 ]
Spanner, M. [10 ]
Ivanov, M. Yu. [11 ]
Smirnova, O. [2 ]
Bauer, D. [12 ]
Popruzhenko, S. V. [13 ]
Vrakking, M. J. J. [1 ,2 ]
机构
[1] FOM Inst AMOLF, NL-1098 XG Amsterdam, Netherlands
[2] Max Born Inst, D-12489 Berlin, Germany
[3] Univ Lyon 1, CNRS, UMR 5579, Spectrometrie Ion & Mol Lab, F-69622 Villeurbanne, France
[4] Univ Toulouse, UPS, Inst Rech Syst Atom & Mol Complexes, Lab Collis, F-31062 Toulouse, France
[5] CNRS, UMR 5589, F-31062 Toulouse, France
[6] Univ Paris 06, CNRS, UMR 7614, Lab Chim Phys Mat & Rayonnement, F-75005 Paris, France
[7] FOM Inst Plasma Phys Rijnhuizen, NL-3439 MN Nieuwegein, Netherlands
[8] SARA Comp & Networking Serv, NL-1098 XG Amsterdam, Netherlands
[9] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA
[10] Natl Res Council Canada, Ottawa, ON K1A 0R6, Canada
[11] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2BW, England
[12] Univ Rostock, Inst Phys, D-18051 Rostock, Germany
[13] Natl Res Nucl Univ, Moscow Engn Phys Inst, Moscow 115409, Russia
基金
英国工程与自然科学研究理事会;
关键词
ABOVE-THRESHOLD IONIZATION; FIELD; DYNAMICS; MOLECULES; RESCATTERING; DIFFRACTION; PHYSICS; RINGS;
D O I
10.1126/science.1198450
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Ionization is the dominant response of atoms and molecules to intense laser fields and is at the basis of several important techniques, such as the generation of attosecond pulses that allow the measurement of electron motion in real time. We present experiments in which metastable xenon atoms were ionized with intense 7-micrometer laser pulses from a free-electron laser. Holographic structures were observed that record underlying electron dynamics on a sublaser-cycle time scale, enabling photoelectron spectroscopy with a time resolution of almost two orders of magnitude higher than the duration of the ionizing pulse.
引用
收藏
页码:61 / 64
页数:4
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