Atmospheric microplastic deposition in an urban environment and an evaluation of transport

被引:711
作者
Wright, S. L. [1 ,2 ]
Ulke, J. [1 ,4 ]
Font, A. [1 ,2 ]
Chan, K. L. A. [3 ]
Kelly, F. J. [1 ,2 ]
机构
[1] Kings Coll London, MRC Ctr Environm & Hlth Analyt Environm & Forens, London, England
[2] Kings Coll London, Environm Res Grp, Analyt Environm & Forens Sci, London, England
[3] Kings Coll London, Sch Canc & Pharmaceut Sci, Inst Pharmaceut Sci, London, England
[4] Univ Potsdam, Inst Nutr Sci, Nuthetal, Germany
基金
英国医学研究理事会; 英国自然环境研究理事会;
关键词
Microplastics; Atmospheric deposition; Air pollution; Urban; POLLUTION; FALLOUT; FIBERS;
D O I
10.1016/j.envint.2019.105411
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Microplastics are a global environmental issue contaminating aquatic and terrestrial environments. They have been reported in atmospheric deposition, and indoor and outdoor air, raising concern for public health due to the potential for exposure. Moreover, the atmosphere presents a new vehicle for microplastics to enter the wider environment, yet our knowledge of the quantities, characteristics and pathways of airborne microplastics is sparse. Here we show microplastics in atmospheric deposition in a major population centre, central London. Microplastics were found in all samples, with deposition rates ranging from 575 to 1008 microplastics/m(2)/d. They were found in various shapes, of which fibrous microplastics accounted for the great majority (92%). Across all samples, 15 different petrochemical-based polymers were identified. Bivariate polar plots indicated dependency on wind, with different source areas for fibrous and non-fibrous airborne microplastics. This is the first evidence of airborne microplastics in London and confirms the need to include airborne pathways when consolidating microplastic impacts on the wider environment and human health.
引用
收藏
页数:7
相关论文
共 36 条
[1]   Atmospheric transport and deposition of microplastics in a remote mountain catchment [J].
Allen, Steve ;
Allen, Deonie ;
Phoenix, Vernon R. ;
Le Roux, Gael ;
Jimenez, Pilar Durantez ;
Simonneau, Anaelle ;
Binet, Stephane ;
Galop, Didier .
NATURE GEOSCIENCE, 2019, 12 (05) :339-+
[2]   The plastic in microplastics: A review [J].
Andrady, Anthony L. .
MARINE POLLUTION BULLETIN, 2017, 119 (01) :12-22
[3]   Boundary layer dynamics over London, UK, as observed using Doppler lidar during REPARTEE-II [J].
Barlow, J. F. ;
Dunbar, T. M. ;
Nemitz, E. G. ;
Wood, C. R. ;
Gallagher, M. W. ;
Davies, F. ;
O'Connor, E. ;
Harrison, R. M. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (05) :2111-2125
[4]   White and wonderful? Microplastics prevail in snow from the Alps to the Arctic [J].
Bergmann, Melanie ;
Muetzel, Sophia ;
Primpke, Sebastian ;
Tekman, Mine B. ;
Trachsel, Jurg ;
Gerdts, Gunnar .
SCIENCE ADVANCES, 2019, 5 (08)
[5]   Characteristic of microplastics in the atmospheric fallout from Dongguan city, China: preliminary research and first evidence [J].
Cai, Liqi ;
Wang, Jundong ;
Peng, Jinping ;
Tan, Zhi ;
Zhan, Zhiwei ;
Tan, Xiangling ;
Chen, Qiuqiang .
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2017, 24 (32) :24928-24935
[6]   openair - An R package for air quality data analysis [J].
Carslaw, David C. ;
Ropkins, Karl .
ENVIRONMENTAL MODELLING & SOFTWARE, 2012, 27-28 :52-61
[7]   Widespread distribution of microplastics in subsurface seawater in the NE Pacific Ocean [J].
Desforges, Jean-Pierre W. ;
Galbraith, Moira ;
Dangerfield, Neil ;
Ross, Peter S. .
MARINE POLLUTION BULLETIN, 2014, 79 (1-2) :94-99
[8]   Synthetic fibers in atmospheric fallout: A source of microplastics in the environment? [J].
Dris, Rachid ;
Gasperi, Johnny ;
Saad, Mohamed ;
Mirande, Cecile ;
Tassin, Bruno .
MARINE POLLUTION BULLETIN, 2016, 104 (1-2) :290-293
[9]   Plastic pollution in Swiss surface waters: nature and concentrations, interaction with pollutants [J].
Faure, Florian ;
Demars, Colin ;
Wieser, Olivier ;
Kunz, Manuel ;
de Alencastro, Luiz Felippe .
ENVIRONMENTAL CHEMISTRY, 2015, 12 (05) :582-591
[10]   Using metal ratios to detect emissions from municipal waste incinerators in ambient air pollution data [J].
Font, Anna ;
de Hoogh, Kees ;
Leal-Sanchez, Maria ;
Ashworth, Danielle C. ;
Brown, Richard J. C. ;
Hansell, Anna L. ;
Fuller, Gary W. .
ATMOSPHERIC ENVIRONMENT, 2015, 113 :177-186