Aggregation and sedimentation of active Brownian particles at constant affinity

被引:15
作者
Fischer, Andreas [1 ,2 ]
Chatterjee, Arkya [3 ]
Speck, Thomas [1 ]
机构
[1] Johannes Gutenberg Univ Mainz, Inst Phys, Staudingerweg 7-9, D-55128 Mainz, Germany
[2] Grad Sch Mat Sci Mainz, Staudinger Weg 9, D-55128 Mainz, Germany
[3] Indian Inst Technol, Dept Phys, Mumbai 400076, India
关键词
EQUATION-OF-STATE; MOTION; MOLECULES; SPHERES;
D O I
10.1063/1.5081115
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We study the motility-induced phase separation of active particles driven through the interconversion of two chemical species controlled by ideal reservoirs (chemostats). As a consequence, the propulsion speed is non-constant and depends on the actual inter-particle forces, enhancing the positive feedback between increased density and reduced motility that is responsible for the observed inhomogeneous density. For hard discs, we find that this effect is negligible and that the phase separation is controlled by the average propulsion speed. For soft particles and large propulsion speeds, however, we predict an observable impact on the collective behavior. We briefly comment on the reentrant behavior found for soft discs. Finally, we study the influence of non-constant propulsion on the sedimentation profile of non-interacting active particles.
引用
收藏
页数:8
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共 55 条
[1]   Self-organization of active particles by quorum sensing rules [J].
Baeuerle, Tobias ;
Fischer, Andreas ;
Speck, Thomas ;
Bechinger, Clemens .
NATURE COMMUNICATIONS, 2018, 9
[2]   PERTURBATION THEORY AND EQUATION OF STATE FOR FLUIDS .2. A SUCCESSFUL THEORY OF LIQUIDS [J].
BARKER, JA ;
HENDERSO.D .
JOURNAL OF CHEMICAL PHYSICS, 1967, 47 (11) :4714-&
[3]   Active Particles in Complex and Crowded Environments [J].
Bechinger, Clemens ;
Di Leonardo, Roberto ;
Loewen, Hartmut ;
Reichhardt, Charles ;
Volpe, Giorgio ;
Volpe, Giovanni .
REVIEWS OF MODERN PHYSICS, 2016, 88 (04)
[4]   Negative Interfacial Tension in Phase-Separated Active Brownian Particles [J].
Bialke, Julian ;
Siebert, Jonathan T. ;
Loewen, Hartmut ;
Speck, Thomas .
PHYSICAL REVIEW LETTERS, 2015, 115 (09)
[5]   Active colloidal suspensions: Clustering and phase behavior [J].
Bialke, Julian ;
Speck, Thomas ;
Loewen, Hartmut .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 2015, 407 :367-375
[6]   Microscopic theory for the phase separation of self-propelled repulsive disks [J].
Bialke, Julian ;
Loewen, Hartmut ;
Speck, Thomas .
EPL, 2013, 103 (03)
[7]   Emergence of macroscopic directed motion in populations of motile colloids [J].
Bricard, Antoine ;
Caussin, Jean-Baptiste ;
Desreumaux, Nicolas ;
Dauchot, Olivier ;
Bartolo, Denis .
NATURE, 2013, 503 (7474) :95-98
[8]   Dynamical Clustering and Phase Separation in Suspensions of Self-Propelled Colloidal Particles [J].
Buttinoni, Ivo ;
Bialke, Julian ;
Kuemmel, Felix ;
Loewen, Hartmut ;
Bechinger, Clemens ;
Speck, Thomas .
PHYSICAL REVIEW LETTERS, 2013, 110 (23)
[9]   Comment on "Entropy Production and Fluctuation Theorems for Active Matter" [J].
Caprini, Lorenzo ;
Marconi, Umberto Marini Bettolo ;
Puglisi, Andrea ;
Vulpiani, Angelo .
PHYSICAL REVIEW LETTERS, 2018, 121 (13)
[10]   Motility-Induced Phase Separation [J].
Cates, Michael E. ;
Tailleur, Julien .
ANNUAL REVIEW OF CONDENSED MATTER PHYSICS, VOL 6, 2015, 6 :219-244