An Mn(V)-oxo role in splitting water?

被引:24
作者
Britt, R. David [1 ]
Suess, Daniel L. M. [1 ]
Stich, Troy A. [1 ]
机构
[1] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA
关键词
OXYGEN-EVOLVING COMPLEX; PHOTOSYSTEM-II; ELECTRONIC-STRUCTURE; SYNTHETIC MODEL; CRYSTAL; CLUSTER;
D O I
10.1073/pnas.1505223112
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
引用
收藏
页码:5265 / 5266
页数:2
相关论文
共 20 条
[1]   The Electronic Structure of the Vanadyl Ion [J].
Ballhausen, C. J. ;
Gray, Harry B. .
INORGANIC CHEMISTRY, 1962, 1 (01) :111-122
[2]   Electronic structure of the oxygenevolving complex in photosystem II prior to O-O bond formation [J].
Cox, Nicholas ;
Retegan, Marius ;
Neese, Frank ;
Pantazis, Dimitrios A. ;
Boussac, Alain ;
Lubitz, Wolfgang .
SCIENCE, 2014, 345 (6198) :804-808
[3]   Biological Water Oxidation [J].
Cox, Nicholas ;
Pantazis, Dimitrios A. ;
Neese, Frank ;
Lubitz, Wolfgang .
ACCOUNTS OF CHEMICAL RESEARCH, 2013, 46 (07) :1588-1596
[4]   Architecture of the photosynthetic oxygen-evolving center [J].
Ferreira, KN ;
Iverson, TM ;
Maghlaoui, K ;
Barber, J ;
Iwata, S .
SCIENCE, 2004, 303 (5665) :1831-1838
[5]   High-spin Mn-oxo complexes and their relevance to the oxygen-evolving complex within photosystem II [J].
Gupta, Rupal ;
Taguchi, Taketo ;
Lassalle-Kaiser, Benedikt ;
Bominaar, Emile L. ;
Yano, Junko ;
Hendrich, Michael P. ;
Borovik, A. S. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2015, 112 (17) :5319-5324
[6]   Photosynthetic O2 formation tracked by time-resolved X-ray experiments [J].
Haumann, M ;
Liebisch, P ;
Müller, C ;
Barra, M ;
Grabolle, M ;
Dau, H .
SCIENCE, 2005, 310 (5750) :1019-1021
[7]   A Synthetic Model of the Mn3Ca Subsite of the Oxygen-Evolving Complex in Photosystem II [J].
Kanady, Jacob S. ;
Tsui, Emily Y. ;
Day, Michael W. ;
Agapie, Theodor .
SCIENCE, 2011, 333 (6043) :733-736
[8]   COOPERATION OF CHARGES IN PHOTOSYNTHETIC O2 EVOLUTION .1. A LINEAR 4STEP MECHANISM [J].
KOK, B ;
FORBUSH, B ;
MCGLOIN, M .
PHOTOCHEMISTRY AND PHOTOBIOLOGY, 1970, 11 (06) :457-&
[9]   A mechanistic and structural model for the formation and reactivity of a MnV=O species in photosynthetic water oxidation [J].
Limburg, J ;
Szalai, VA ;
Brudvig, GW .
JOURNAL OF THE CHEMICAL SOCIETY-DALTON TRANSACTIONS, 1999, (09) :1353-1361
[10]   SYNTHESIS, REACTIONS, AND ELECTRONIC-STRUCTURE OF LOW-VALENT RHENIUM-OXO COMPOUNDS - CRYSTAL AND MOLECULAR-STRUCTURE OF RE(O)I(MEC=CME)2 [J].
MAYER, JM ;
THORN, DL ;
TULIP, TH .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1985, 107 (25) :7454-7462