Efficient conversion of methane into power via microchanneled solid oxide fuel cells

被引:16
作者
Wang, Jingjing [1 ]
Fan, Dongjie [1 ]
Yu, Libo [1 ]
Wei, Tao [1 ]
Hu, Xun [1 ]
Ye, Zhengmao [1 ]
Wang, Zhi [1 ]
Wang, Yi [2 ]
Li, Cuncheng [3 ]
Yao, Jianfeng [4 ]
Dong, Dehua [1 ]
机构
[1] Univ Jinan, Sch Mat Sci & Engn, Jinan 250022, Peoples R China
[2] Huazhong Univ Sci & Technol, Sch Energy & Power Engn, Wuhan 430074, Peoples R China
[3] Univ Jinan, Sch Chem & Chem Engn, Jinan 250022, Peoples R China
[4] Nanjing Forestry Univ, Coll Chem Engn, Jiangsu Key Lab Chem & Utilizat Agr & Forest Biom, Nanjing 210037, Peoples R China
基金
中国国家自然科学基金;
关键词
Methane-fueled SOFCs; Methane conversion efficiency; Gas diffusion; Anode supports; Microchannel structure; ELECTROLYSIS CELLS; CO2; ELECTROLYSIS; DIRECT OPERATION; ANODE; CARBON; SOFCS; DEPOSITION; SUPPORT;
D O I
10.1016/j.jpowsour.2020.227848
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Methane-fueled solid oxide fuel cells (SOFCs) are promising to achieve high energy conversion efficiency while no study focuses on the conversion efficiency of methane into power, which is greatly restrained by gas diffusion within anode supports. This study employs microchanneled anode supports to provide fast gas diffusion pathway. To confirm the advantage, the anodes with half-channels and without channels are also used for comparison. The microchannel structure increases the maximum power density up to 2.5 times because of diminishing or eliminating concentration polarization within anode supports and improving catalyst coating over anode internal surface. As a compromise of fuel utilization and power output, methane conversion efficiency is defined as power output per mol methane input in feeding gas to compare with the reported results, and the microchanneled SOFCs achieve the record high methane conversion efficiency.
引用
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页数:6
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