An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds

被引：314

作者：

Kolb, C. E. ^{[1
]}

Cox, R. A. ^{[2
]}

Abbatt, J. P. D. ^{[3
]}

Ammann, M. ^{[4
]}

Davis, E. J. ^{[5
]}

Donaldson, D. J. ^{[3
]}

Garrett, B. C. ^{[6
]}

George, C. ^{[7
]}

Griffiths, P. T. ^{[2
]}

Hanson, D. R. ^{[8
]}

Kulmala, M. ^{[9
]}

McFiggans, G. ^{[10
]}

Poeschl, U. ^{[11
]}

Riipinen, I. ^{[9
]}

Rossi, M. J. ^{[12
]}

Rudich, Y. ^{[13
]}

Wagner, P. E. ^{[14
]}

Winkler, P. M. ^{[14
,15
]}

Worsnop, D. R. ^{[1
,9
]}

O'Dowd, C. D. ^{[16
,17
]}

机构：

[1] Aerodyne Res Inc, Ctr Aerosol & Cloud Chem, Billerica, MA 01821 USA

[2] Univ Cambridge, Ctr Atmospher Sci, Dept Chem, Cambridge CB2 1EP, England

[3] Univ Toronto, Dept Chem, Toronto, ON M5S 3H6, Canada

[4] Paul Scherrer Inst, Lab Radiochem & Environm Chem, CH-5232 Villigen, Switzerland

[5] Univ Washington, Dept Chem Engn, Seattle, WA 98195 USA

[6] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA

[7] Univ Lyon 1 2, IRCELYON, Inst Rech Catalyse & Environm Lyon, CNRS UMR 5256, F-69626 Villeurbanne, France

[8] Augsburg Coll, Minneapolis, MN 55454 USA

[9] Univ Helsinki, Dept Phys Sci, FIN-00014 Helsinki, Finland

[10] Univ Manchester, Ctr Atmospher Sci, Sch Earth Atmospher & Environm Sci, Manchester M13 9PL, Lancs, England

[11] Max Planck Inst Chem, Biogeochem Dept, D-55128 Mainz, Germany

[12] Paul Scherrer Inst, Lab Atmosphaerenchem, OFLA008, CH-5232 Villigen, Switzerland

[13] Weizmann Inst Sci, Dept Environm Sci, IL-76100 Rehovot, Israel

[14] Univ Vienna, Fac Phys, A-1090 Vienna, Austria

[15] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80305 USA

[16] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland

[17] Natl Univ Ireland Galway, Ctr Climate & Air Pollut Studies, Galway, Ireland

来源：

ATMOSPHERIC CHEMISTRY AND PHYSICS | 2010年 / 10卷 / 21期

关键词：

LIQUID-VAPOR INTERFACE; MASS ACCOMMODATION COEFFICIENT; MOLECULAR-DYNAMICS SIMULATIONS; AIR-WATER-INTERFACE; UNSATURATED FATTY-ACIDS; TRANSITION-STATE THEORY; HETEROGENEOUS CHEMICAL-KINETICS; REACTIVE UPTAKE COEFFICIENTS; SURFACE-TENSION MEASUREMENTS; DROPLET GROWTH-KINETICS;

D O I：

10.5194/acp-10-10561-2010

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

A workshop was held in the framework of the ACCENT (Atmospheric Composition Change - a European Network) Joint Research Programme on "Aerosols" and the Programme on "Access to Laboratory Data". The aim of the workshop was to hold "Gordon Conference" type discussion covering accommodation and reactive uptake of water vapour and trace pollutant gases on condensed phase atmospheric materials. The scope was to review and define the current state of knowledge of accommodation coefficients for water vapour on water droplet and ice surfaces, and uptake of trace gas species on a variety of different surfaces characteristic of the atmospheric condensed phase particulate matter and cloud droplets. Twenty-six scientists participated in this meeting through presentations, discussions and the development of a consensus review. In this review we present an analysis of the state of knowledge on the thermal and mass accommodation coefficient for water vapour on aqueous droplets and ice and a survey of current state-of the-art of reactive uptake of trace gases on a range of liquid and solid atmospheric droplets and particles. The review recommends consistent definitions of the various parameters that are needed for quantitative representation of the range of gas/condensed surface kinetic processes important for the atmosphere and identifies topics that require additional research.

引用

页码：10561 / 10605

页数：45

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