Room-Temperature Voltage Tunable Phonon Thermal Conductivity via Reconfigurable Interfaces in Ferroelectric Thin Films

被引:150
作者
Ihlefeld, Jon F. [1 ]
Foley, Brian M. [2 ]
Scrymgeour, David A. [1 ]
Michael, Joseph R. [1 ]
McKenzie, Bonnie B. [1 ]
Medlin, Douglas L. [3 ]
Wallace, Margeaux [4 ]
Trolier-McKinstry, Susan [4 ]
Hopkins, Patrick E. [2 ]
机构
[1] Sandia Natl Labs, Albuquerque, NM 87185 USA
[2] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA
[3] Sandia Natl Labs, Livermore, CA 94550 USA
[4] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA
基金
美国国家科学基金会; 美国能源部;
关键词
Thermal conductivity; tunable; time domain thermoreflectance; ferroelectric; nano domain; ELECTRIC-FIELD; DOMAIN-WALLS; HEAT-FLOW; TRANSPORT; CERAMICS; DYNAMICS; KH2PO4; STATE;
D O I
10.1021/nl504505t
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Dynamic control of thermal transport in solid-state systems is a transformative capahility with the promise to propel technologies including phonornt-logic, thermal managernent, and energy harvesting. A solid-state solution to rapidly manipulate phonons has escaped the scientific corrithuriity. We demonstrate active and reversible tuning of thermal conductivity by manipulating the nanoScale ferroelastic domain structure of a Pb(Zr0.3Ti0.7)O-3 film with applied electric fields. With subsecond response times, the room-temperature thermal conductivity was modulated by 11%.
引用
收藏
页码:1791 / 1795
页数:5
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