Toward Efficient Orange Emissive Carbon Nanodots through Conjugated sp2-Domain Controlling and Surface Charges Engineering

被引:648
作者
Qu, Songnan [1 ]
Zhou, Ding [1 ]
Li, Di [1 ]
Ji, Wenyu [1 ]
Jing, Pengtao [1 ]
Han, Dong [1 ]
Liu, Lei [1 ]
Zeng, Haibo [2 ]
Shen, Dezhen [1 ]
机构
[1] Chinese Acad Sci, Changchun Inst Opt Fine Mech & Phys, State Key Lab Luminescence & Applicat, 3888 Eastern South Lake Rd, Changchun 130033, Jilin, Peoples R China
[2] Nanjing Univ Sci & Technol, Coll Mat Sci & Engn, Inst Optoelect & Nanomat, Nanjing 210094, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
GRAPHENE QUANTUM DOTS; LIGHT-EMITTING-DIODES; LUMINESCENCE; GREEN;
D O I
10.1002/adma.201504891
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A strategy of achieving efficient orange emissive carbon nanodots (CNDs) with large sized conjugated sp(2)-domain is achieved in a solvothermal synthetic route using dimethylformamide as solvent, which is the basis of orange bandgap emission; enhanced orange emission with photoluminescent quantum yield of 46% is realized through surface charges engineering by surface metal-cation-functionalization.
引用
收藏
页码:3516 / +
页数:7
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