A new index for precise design and advanced operation of mass transfer in slug flow

被引:50
作者
Aoki, Nobuaki [1 ]
Tanigawa, Shin [1 ]
Mae, Kazuhiro [1 ]
机构
[1] Kyoto Univ, Grad Sch Engn, Dept Chem Engn, Nishikyo Ku, Kyoto 6158510, Japan
关键词
Slug flow; Microchannel; Mass transfer; Internal circulation flow; Sudden expansion; LIQUID SLUGS; MICROREACTOR; MICROCHANNEL; EXTRACTION; CAPILLARY; SYSTEMS;
D O I
10.1016/j.cej.2010.07.071
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Slug flow, one of the ordered multi-phase flow patterns in a small channel, has the advantage of the enhancement of mixing in each phase and mass transfer between two phases due to the internal circulation flow. To form stable slug flow, the throughput of order of mu L min(-1) has been employed. To use slug flow in industrial scale, however, controlled and high throughput mass transfer and an index for design of a channel with slug flow are required. To address this requirement, we examined the influences of operating conditions such as the channel size and the flow rate on flow patterns and the mass transfer rate. Based on the experimental results, we derived an index to represent the mass transfer rate in slug flow. For further improvement of mass transfer in slug flow, we also verified that the channel including a sudden expansion improves the mass transfer efficiency. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:651 / 656
页数:6
相关论文
共 12 条
[1]  
Arirachakaran S., 1989, 18836 SPE, P155
[2]   The intensification of rapid reactions in multiphase systems using slug flow in capillaries [J].
Burns, JR ;
Ramshaw, C .
LAB ON A CHIP, 2001, 1 (01) :10-15
[3]  
Charles M.E., 1961, CAN J CHEM ENG, V39, P27, DOI DOI 10.1002/CJCE.5450390106
[4]   CFD modelling of mass transfer with and without chemical reaction in the liquid-liquid slug flow microreactor [J].
Kashid, M. N. ;
Agar, D. W. ;
Turek, S. .
CHEMICAL ENGINEERING SCIENCE, 2007, 62 (18-20) :5102-5109
[5]   Liquid-liquid slug flow in a capillary: An alternative to suspended drop or film contactors [J].
Kashid, M. N. ;
Harshe, Y. M. ;
Agar, D. W. .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2007, 46 (25) :8420-8430
[6]   Internal circulation within the liquid slugs of a liquid-liquid slug-flow capillary microreactor [J].
Kashid, MN ;
Gerlach, I ;
Goetz, S ;
Franzke, J ;
Acker, JF ;
Platte, F ;
Agar, DW ;
Turek, S .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2005, 44 (14) :5003-5010
[7]   THE EFFECT OF GAS INJECTION ON THE FLOW OF IMMISCIBLE LIQUIDS IN HORIZONTAL PIPES [J].
NADLER, M ;
MEWES, D .
CHEMICAL ENGINEERING & TECHNOLOGY, 1995, 18 (03) :156-165
[8]   Effect of alternating pumping of two reactants into a microchannel on a phase transfer reaction [J].
Okamoto, H .
CHEMICAL ENGINEERING & TECHNOLOGY, 2006, 29 (04) :504-506
[9]   Microchannel devices for the coalescence of dispersed droplets produced for use in rapid extraction processes [J].
Okubo, Y ;
Toma, M ;
Ueda, H ;
Maki, T ;
Mae, K .
CHEMICAL ENGINEERING JOURNAL, 2004, 101 (1-3) :39-48
[10]   Liquid-liquid extraction for efficient synthesis and separation by utilizing micro spaces [J].
Okubo, Yoshihito ;
Maki, Taisuke ;
Aoki, Nobuaki ;
Khoo, Teng Hong ;
Ohmukai, Yoshikage ;
Mae, Kazuhiro .
CHEMICAL ENGINEERING SCIENCE, 2008, 63 (16) :4070-4077