Relay transport of aerosols to Beijing-Tianjin-Hebei region by multi-scale atmospheric circulations

被引:82
作者
Miao, Yucong [1 ]
Guo, Jianping [1 ]
Liu, Shuhua [2 ]
Liu, Huan [1 ]
Zhang, Gen [1 ,3 ]
Yan, Yan [1 ]
He, Jing [1 ]
机构
[1] Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China
[2] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Beijing 100871, Peoples R China
[3] Shanghai Key Lab Meteorol & Hlth, Shanghai 200135, Peoples R China
基金
中国国家自然科学基金;
关键词
Beijing-Tianjin-Hebei region; Sea-breeze; Aerosol pollution; WRF-chem; Trans-boundary transport; BOUNDARY-LAYER STRUCTURE; NORTH CHINA PLAIN; AIR-QUALITY; SEVERE HAZE; SOURCE APPORTIONMENT; WINTER HAZE; POLLUTION; PM2.5; MODEL; MECHANISM;
D O I
10.1016/j.atmosenv.2017.06.032
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The Beijing-Tianjin-Hebei (BTH) region experiences heavy aerosol pollution, which is found to have close relationships with the synoptic- and local-scale atmospheric circulations. However, how and to what extent these multi-scale circulations interplay to modulate aerosol transport have not been fully understood. To this end, this study comprehensively investigated the impacts of these circulations on aerosol transport in BTH by focusing on an episode occurred on 1 June 2013 through combining both observations and three-dimensional simulations. It was found that during this episode, the Bohai Sea acted as a transfer station, and the high-pressure system over the Yellow Sea and sea-breeze in BTH took turns to affect the transport of aerosols. In the morning, influenced by the high-pressure system, lots of aerosols emitted from Shandong and Jiangsu provinces were first transported to the Bohai Sea. After then, these aerosols were brought to the BTH region in the afternoon through the inland penetration of sea-breeze, significantly exacerbating the air quality in BTH. The inland penetration of sea-breeze could be identified by the sharp changes in ground-based observed temperature, humidity, and wind when the sea-breeze front (SBF) passed by. Combining observations with model outputs, the SBF was found to be able to advance inland more than similar to 150 km till reaching Beijing. This study has important implications for better understanding the aerosol transport in BTH, and improving the forecast of such aerosol pollution. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:35 / 45
页数:11
相关论文
共 59 条
[1]   Modal aerosol dynamics model for Europe: Development and first applications [J].
Ackermann, IJ ;
Hass, H ;
Memmesheimer, M ;
Ebel, A ;
Binkowski, FS ;
Shankar, U .
ATMOSPHERIC ENVIRONMENT, 1998, 32 (17) :2981-2999
[2]  
BANTA R, 1981, J APPL METEOROL, V20, P1255, DOI 10.1175/1520-0450(1981)020<1255:AAOTSO>2.0.CO
[3]  
2
[4]   Air pollution in mega cities in China [J].
Chan, Chak K. ;
Yao, Xiaohong .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (01) :1-42
[5]  
Chen F, 2001, MON WEATHER REV, V129, P569, DOI 10.1175/1520-0493(2001)129<0569:CAALSH>2.0.CO
[6]  
2
[7]   Modeling temporal variations in global residential energy consumption and pollutant emissions [J].
Chen, Han ;
Huang, Ye ;
Shen, Huizhong ;
Chen, Yilin ;
Ru, Muye ;
Chen, Yuanchen ;
Lin, Nan ;
Su, Shu ;
Zhuo, Shaojie ;
Zhong, Qirui ;
Wang, Xilong ;
Liu, Junfeng ;
Li, Bengang ;
Tao, Shu .
APPLIED ENERGY, 2016, 184 :820-829
[8]   The ERA-Interim reanalysis: configuration and performance of the data assimilation system [J].
Dee, D. P. ;
Uppala, S. M. ;
Simmons, A. J. ;
Berrisford, P. ;
Poli, P. ;
Kobayashi, S. ;
Andrae, U. ;
Balmaseda, M. A. ;
Balsamo, G. ;
Bauer, P. ;
Bechtold, P. ;
Beljaars, A. C. M. ;
van de Berg, L. ;
Bidlot, J. ;
Bormann, N. ;
Delsol, C. ;
Dragani, R. ;
Fuentes, M. ;
Geer, A. J. ;
Haimberger, L. ;
Healy, S. B. ;
Hersbach, H. ;
Holm, E. V. ;
Isaksen, L. ;
Kallberg, P. ;
Koehler, M. ;
Matricardi, M. ;
McNally, A. P. ;
Monge-Sanz, B. M. ;
Morcrette, J. -J. ;
Park, B. -K. ;
Peubey, C. ;
de Rosnay, P. ;
Tavolato, C. ;
Thepaut, J. -N. ;
Vitart, F. .
QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY, 2011, 137 (656) :553-597
[9]   Improving simulations of sulfate aerosols during winter haze over Northern China: the impacts of heterogeneous oxidation by NO2 [J].
Gao, Meng ;
Carmichael, Gregory R. ;
Wang, Yuesi ;
Ji, Dongsheng ;
Liu, Zirui ;
Wang, Zifa .
FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING, 2016, 10 (05)
[10]   Emission controls versus meteorological conditions in determining aerosol concentrations in Beijing during the 2008 Olympic Games [J].
Gao, Y. ;
Liu, X. ;
Zhao, C. ;
Zhang, M. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (23) :12437-12451