Enhanced light extraction from organic light emitting diodes using a flexible polymer-nanoparticle scattering layer

被引:16
作者
Sajeev, Anjali K. [1 ,2 ]
Agarwal, Nishkarsh [3 ]
Soman, Anjaly [1 ,2 ]
Gupta, Shilpi [4 ]
Katiyar, Monica [3 ]
Ajayaghosh, A. [1 ,2 ]
Unni, K. N. Narayanan [1 ,2 ]
机构
[1] CSIR Natl Inst Interdisciplinary Sci & Technol CS, Chem Sci & Technol Div, Photosci & Photon Sect, Thiruvananthapuram 695019, Kerala, India
[2] Acad Sci & Innovat Res AcSIR, Ghaziabad 201002, India
[3] Indian Inst Technol Kanpur, Dept Mat Sci & Engn, Kanpur 208016, Uttar Pradesh, India
[4] Indian Inst Technol Kanpur, Dept Elect Engn, Kanpur 208016, Uttar Pradesh, India
关键词
OLED; Optical outcoupling; Mie scattering; External light extraction; OUTCOUPLING ENHANCEMENT; REFRACTIVE-INDEX; EFFICIENCY; DEVICES; EMISSION; ELECTROLUMINESCENCE; IMPROVEMENT; FABRICATION; PATTERN; FILMS;
D O I
10.1016/j.orgel.2021.106386
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Efficient optical outcoupling from organic light emitting diodes (OLEDs) is an important challenge in solid state lighting technology. In this work, the effect of an external light extraction layer, prepared using polydimethylsiloxane (PDMS) and zinc oxide (ZnO) nanoparticles, was studied on the performance of red, green, blue and white OLEDs. The self-standing flexible film can effectively address the loss modes at the substrate-air interface. With the application of the layer, a maximum enhancement of about 80% in light outcoupling was observed in white OLEDs. Monochrome OLEDs also showed appreciable enhancement in emission with green having the highest improvement (102%), followed by red (56%) and blue (35%). Finite-difference time-domain (FDTD) simulations were performed for elucidating the mechanism behind the improvement in light extraction due to nanoparticle scattering layer. Total-Field Scattered-Field (TFSF) source was used to simulate the scattering cross-section for different wavelengths. Reduced Fresnel reflections at the air-glass interface and advantageous Mie scattering by ZnO nanoparticles seem to increase the optical outcoupling. This film could be a potential candidate for light extraction in OLEDs because of its facile fabrication, economical precursors, and adaptability to flexible substrates and absence of any possible optical artefacts to the emission.
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页数:11
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共 66 条
[1]   Nearly 100% internal phosphorescence efficiency in an organic light-emitting device [J].
Adachi, C ;
Baldo, MA ;
Thompson, ME ;
Forrest, SR .
JOURNAL OF APPLIED PHYSICS, 2001, 90 (10) :5048-5051
[2]   Functional inorganic nanofillers for transparent polymers [J].
Althues, H. ;
Henle, J. ;
Kaskel, S. .
CHEMICAL SOCIETY REVIEWS, 2007, 36 (09) :1454-1465
[3]   Fabrication of the dispersed hollow polymer scattering layer for enhancing the light out-coupling of organic light-emitting diodes [J].
Ban, Uk Hyeon ;
Kim, Dong Woo ;
Han, Joo Won ;
Kim, Yong Hyun ;
Park, Chan ;
Gal, Yeong-Soon ;
Lim, Kwon Taek .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 2018, 663 (01) :182-189
[4]   Bottom-up honeycomb top layer for light outcoupling enhancement in blue organic light emitting diodes [J].
Bertrand, A. ;
Dumur, F. ;
Mruczkiewicz, M. ;
Perrin, M. ;
Lartigau-Dagron, C. ;
Bousquet, A. ;
Vignau, L. ;
Billon, L. ;
Fasquel, S. .
ORGANIC ELECTRONICS, 2018, 52 :222-229
[5]   White organic light emitting diodes with enhanced internal and external outcoupling for ultra-efficient light extraction and Lambertian emission [J].
Bocksrocker, Tobias ;
Preinfalk, Jan Benedikt ;
Asche-Tauscher, Julian ;
Pargner, Andreas ;
Eschenbaum, Carsten ;
Maier-Flaig, Florian ;
Lemmer, Uli .
OPTICS EXPRESS, 2012, 20 (23) :A932-A940
[6]   Weak microcavity effects in organic light-emitting devices [J].
Bulovic, V ;
Khalfin, VB ;
Gu, G ;
Burrows, PE ;
Garbuzov, DZ ;
Forrest, SR .
PHYSICAL REVIEW B, 1998, 58 (07) :3730-3740
[7]   Characterization on polystyrene/zinc oxide nanocomposites prepared from solution mixing [J].
Chae, DW ;
Kim, BC .
POLYMERS FOR ADVANCED TECHNOLOGIES, 2005, 16 (11-12) :846-850
[8]   Fourfold power efficiency improvement in organic light-emitting devices using an embedded nanocomposite scattering layer [J].
Chang, Chih-Hao ;
Chang, Kuo-Yan ;
Lo, Yu-Jhong ;
Chang, Shu-Jing ;
Chang, Hsin-Hua .
ORGANIC ELECTRONICS, 2012, 13 (06) :1073-1080
[9]   Nano-particle based scattering layers for optical efficiency enhancement of organic light-emitting diodes and organic solar cells [J].
Chang, Hong-Wei ;
Lee, Jonghee ;
Hofmann, Simone ;
Kim, Yong Hyun ;
Mueller-Meskamp, Lars ;
Luessem, Bjoern ;
Wu, Chung-Chih ;
Leo, Karl ;
Gather, Malte C. .
JOURNAL OF APPLIED PHYSICS, 2013, 113 (20)
[10]   Organic light-emitting devices integrated with internal scattering layers for enhancing optical out-coupling [J].
Chang, Hong-Wei ;
Tien, Kun-Cheng ;
Hsu, Min-Hung ;
Huang, Yi-Hsiang ;
Lin, Ming-Shiang ;
Tsai, Chih-Hung ;
Tsai, Yu-Tang ;
Wu, Chung-Chih .
JOURNAL OF THE SOCIETY FOR INFORMATION DISPLAY, 2011, 19 (02) :196-204