Aggregation-Induced Emission and Retention of Crystal Chiral Information of Tetraphenylethylene Incorporated by Polysaccharides in Water

被引：13
作者：
Hino, Shodai [1 ]
Sugikawa, Kouta [1 ]
Kawasaki, Riku [1 ]
Funabashi, Hisakage [2 ]
Kuroda, Akio [2 ]
Ikeda, Atsushi [1 ]
机构：
[1] Hiroshima Univ, Grad Sch Engn, Dept Appl Chem, 1-4-1 Kagamiyama, Higashihiroshima, Hiroshima 7398527, Japan
[2] Hiroshima Univ, Grad Sch Engn, Dept Mol Biotechnol, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 7398530, Japan
来源：
CHEMPHOTOCHEM | 2020年 / 4卷 / 08期
关键词：
Aggregation; chirality; fluorescent probes; host-guest systems; polysaccharides; WALLED CARBON NANOTUBES; ONE-DIMENSIONAL HOST; PHOTODYNAMIC ACTIVITIES; SOLUBILIZATION; SCHIZOPHYLLAN; FLUORESCENT; SENSORS; BETA-1,3-GLUCAN; DERIVATIVES; ADSORPTION;
D O I：
10.1002/cptc.202000022
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Polysaccharides, such as pullulan and lambda-carrageenan, can incorporate tetraphenylethylene derivatives through self-aggregation in water by a high-speed vibration milling method, which cannot be done by sonication and heating methods. Aggregation-induced emission is observed from the tetraphenylethylene-polysaccharide complexes. Furthermore, the tetraphenylethylene self-assembled into polysaccharides is able to preserve the initial helical chirality (M- or P-helicity) of the crystals in water after ball milling. Intracellular uptake of the polysaccharide-complexed tetraphenylethylene derivative with a phenol unit by HeLa cells is enhanced compared with that without the phenol unit.
引用
收藏
页码：577 / 581
页数：5
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