Bottom-Up Synthesized All-Thermal-Catalyst Aerogels for Heat-Regenerative Air Filtration

被引:9
作者
Ji, Xiang [1 ]
Zhao, Jiayuan [1 ]
Jung, Sung Mi [12 ]
Hrdina, Amy I. H. [2 ,3 ]
Wolf, Martin J. [4 ]
Yang, Xiulin [5 ]
Vaartstra, Geoffrey [6 ]
Xie, Helen [7 ,8 ]
Luo, Shao-Xiong Lennon [9 ,10 ]
Lu, Ang-Yu [1 ]
Welsch, Roy E. [7 ,8 ]
Wang, Evelyn N. [6 ]
Li, Lain-Jong [5 ,11 ]
Kong, Jing [1 ]
机构
[1] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA
[2] MIT, Dept Civil & Environm Engn, Cambridge, MA 02139 USA
[3] MIT, Dept Chem Engn, Cambridge, MA 02139 USA
[4] MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USA
[5] King Abdullah Univ Sci & Technol, Phys Sci & Engn Div, Thuwal 239556900, Saudi Arabia
[6] MIT, Dept Mech Engn, Cambridge, MA 02139 USA
[7] MIT, Sloan Sch Management, Cambridge, MA 02139 USA
[8] MIT, Ctr Stat & Data Sci, Cambridge, MA 02139 USA
[9] MIT, Dept Chem, Cambridge, MA 02139 USA
[10] MIT, Inst Soldier Nanotechnol, Cambridge, MA 02139 USA
[11] Univ Hong Kong, Dept Mech Engn, Pokfulam, Hong Kong, Peoples R China
[12] Korea Inst Toxicol, Environm Fate & Exposure Res Grp, Gyeongnam 52834, South Korea
基金
新加坡国家研究基金会;
关键词
air pollution; all-thermal-catalyst aerogel; heat-regenerative air filter; POLLUTION; PERMEABILITY; STABILITY; REMOVAL;
D O I
10.1021/acs.nanolett.1c02593
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Airborne particular matter (PM) pollution is an increasing global issue and alternative sources of filter fibers are now an area of significant focus. Compared with relatively mature hazardous gas treatments, state of the art high-efficiency PM filters still lack thermal decomposition ability for organic PM pollutants, such as soot from coal-fired power plants and waste-combustion incinerators, resulting in frequent replacement, high cost, and second-hand pollution. In this manuscript, we propose a bottom-up synthesis method to make the first all- thermal-catalyst air filter (ATCAF). Self-assembled from similar to 50 nm diameter TiO2 fibers, ATCAF could not only capture the combustion-generated PM pollutants with >99.999% efficiency but also catalyze the complete decomposition of the as-captured hydrocarbon pollutants at high temperature. It has the potential of in situ eliminating the PM pollutants from burning of hydrocarbon materials leveraging the burning heat.
引用
收藏
页码:8160 / 8165
页数:6
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