A reconfigurable and magnetically responsive assembly for dynamic solar steam generation

被引:120
作者
Hu, Yajie [1 ,2 ]
Ma, Hongyun [1 ,2 ]
Wu, Mingmao [1 ,2 ]
Lin, Tengyu [1 ,2 ,3 ]
Yao, Houze [1 ,2 ]
Liu, Feng [4 ]
Cheng, Huhu [1 ,2 ]
Qu, Liangti [1 ,2 ]
机构
[1] Tsinghua Univ, Key Lab Organ Optoelect & Mol Engn, Minist Educ, Dept Chem,Dept Mech Engn, Beijing 100084, Peoples R China
[2] Tsinghua Univ, State Key Lab Tribol, Dept Mech Engn, Beijing 100084, Peoples R China
[3] HurRain Nano Technol Co Ltd, Beijing 100084, Peoples R China
[4] Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China
基金
美国国家科学基金会;
关键词
EFFICIENCY; GRAPHENE;
D O I
10.1038/s41467-022-32051-3
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Interfacial solar vapor generation is a promising technique to efficiently get fresh water from seawater or effluent. However, for the traditional static evaporation models, further performance improvement has encountered bottlenecks due to the lack of dynamic management and self-regulation on the evolving water movement and phase change in the evaporation process. Here, a reconfigurable and magnetically responsive evaporator with conic arrays is developed through the controllable and reversible assembly of graphene wrapped Fe3O4 nanoparticles. Different from the traditional structure-rigid evaporation architecture, the deformable and dynamic assemblies could reconfigure themselves both at macroscopic and microscopic scales in response to the variable magnetic field. Thus, the internal water transportation and external vapor diffusion are greatly promoted simultaneously, leading to a 23% higher evaporation rate than that of static counterparts. Further, well-designed hierarchical assembly and dynamic evaporation system can boost the evaporation rate to a record high level of 5.9 kg m(-2) h(-1). This proof-of-concept work demonstrates a new direction for development of high performance water evaporation system with the ability of dynamic reconfiguration and reassembly. Despite a promising water harvesting approach solar steam generation low efficiency remains a challenging obstacle. Here, authors present a macro- and microscopically reconfigurable and magnetically responsive assembly towards a dynamic evaporation system with improved performance and salt resistance.
引用
收藏
页数:12
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