Construction of hierarchical-porous metal-organic frameworks through esterification reaction for efficient catalysis

被引:6
作者
Wang, Peng [1 ,2 ,3 ]
Zhang, Peng [1 ,2 ]
Shen, Yu [1 ,2 ]
Wang, Liu [1 ,2 ]
Li, Hongfeng [1 ,2 ]
Zhang, Wenlei [3 ]
Gu, Zhida [3 ]
Zhang, Xinglong [1 ,2 ]
Fu, Yu [3 ]
Zhang, Weina [1 ,2 ]
Huo, Fengwei [1 ,2 ]
机构
[1] Nanjing Tech Univ NanjingTech, Key Lab Flexible Elect KLOFE, 30 South Puzhu Rd, Nanjing 211816, Peoples R China
[2] Nanjing Tech Univ NanjingTech, Inst Adv Mat IAM, 30 South Puzhu Rd, Nanjing 211816, Peoples R China
[3] Northeastern Univ, Coll Sci, Shenyang 100819, Peoples R China
基金
中国国家自然科学基金;
关键词
STRATEGY; HOLLOW; SIZE; MOFS;
D O I
10.1039/d1cc03059k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A solvent-assisted strategy was proposed by controlling the coordination equilibrium to fabricate hierarchical-porous metal-organic frameworks (HP-MOFs). The obtained HP-MOFs showed remarkable enhancement in catalytic efficiency in Lewis acid catalysis resulting from the joint efforts of the hierarchical pores and the exposed metal clusters.
引用
收藏
页码:10795 / 10798
页数:4
相关论文
共 28 条
  • [11] Metal-organic frameworks with catalytic centers: From synthesis to catalytic application
    Kang, Yan-Shang
    Lu, Yi
    Chen, Kai
    Zhao, Yue
    Wang, Peng
    Sun, Wei-Yin
    [J]. COORDINATION CHEMISTRY REVIEWS, 2019, 378 : 262 - 280
  • [12] Hydrolytic Transformation of Microporous Metal-Organic Frameworks to Hierarchical Micro- and Mesoporous MOFs
    Kim, Yonghwi
    Yang, Tao
    Yun, Gyeongwon
    Ghasemian, Mohammad Bagher
    Koo, Jaehyoung
    Lee, Eunsung
    Cho, Sung June
    Kim, Kimoon
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2015, 54 (45) : 13273 - 13278
  • [13] Hollowing out MOFs: hierarchical micro- and mesoporous MOFs with tailorable porosity via selective acid etching
    Koo, Jaehyoung
    Hwang, In-Chul
    Yu, Xiujun
    Saha, Subhadeep
    Kim, Yonghwi
    Kim, Kimoon
    [J]. CHEMICAL SCIENCE, 2017, 8 (10) : 6799 - 6803
  • [14] Multiresponsive Graphene-Aerogel-Directed Phase-Change Smart Fibers
    Li, Guangyong
    Hong, Guo
    Dong, Dapeng
    Song, Wenhui
    Zhang, Xuetong
    [J]. ADVANCED MATERIALS, 2018, 30 (30)
  • [15] Crystal-Growth-Dominated Fabrication of Metal-Organic Frameworks with Orderly Distributed Hierarchical Porosity
    Li, Hang
    Meng, Fanchen
    Zhang, Suoying
    Wang, Liguang
    Li, Matthew
    Ma, Lu
    Zhang, Weina
    Zhang, Wenlei
    Yang, Zhuhong
    Wu, Tianpin
    Lee, Sungsik
    Huo, Fengwei
    Lu, Jun
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2020, 59 (06) : 2457 - 2464
  • [16] Multi-shelled Hollow Metal-Organic Frameworks
    Liu, Wenxian
    Huang, Jijiang
    Yang, Qiu
    Wang, Shiji
    Sun, Xiaoming
    Zhang, Weina
    Liu, Junfeng
    Huo, Fengwei
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (20) : 5512 - 5516
  • [17] Molecular Encapsulation beyond the Aperture Size Limit through Dissociative Linker Exchange in Metal-Organic Framework Crystals
    Morabito, Joseph V.
    Chou, Lien-Yang
    Li, Zhehui
    Manna, Cesar M.
    Petroff, Christopher A.
    Kyada, Rutvin J.
    Palomba, Joseph M.
    Byers, Jeffery A.
    Tsung, Chia-Kuang
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2014, 136 (36) : 12540 - 12543
  • [18] Generation of Hierarchical Porosity in Metal-Organic Frameworks by the Modulation of Cation Valence
    Qi, Shi-Chao
    Qian, Xin-Yu
    He, Qiu-Xia
    Miao, Kang-Jing
    Jiang, Yao
    Tan, Peng
    Liu, Xiao-Qin
    Sun, Lin-Bing
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2019, 58 (30) : 10104 - 10109
  • [19] Hierarchically Micro- and Mesoporous Metal-Organic Frameworks with Tunable Porosity
    Qiu, Ling-Guang
    Xu, Tao
    Li, Zong-Qun
    Wang, Wei
    Wu, Yun
    Jiang, Xia
    Tian, Xing-You
    Zhang, Li-De
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (49) : 9487 - 9491
  • [20] Applications of hierarchically structured porous materials from energy storage and conversion, catalysis, photocatalysis, adsorption, separation, and sensing to biomedicine
    Sun, Ming-Hui
    Huang, Shao-Zhuan
    Chen, Li-Hua
    Li, Yu
    Yang, Xiao-Yu
    Yuan, Zhong-Yong
    Su, Bao-Lian
    [J]. CHEMICAL SOCIETY REVIEWS, 2016, 45 (12) : 3479 - 3563