A triad [FeFe] hydrogenase system for light-driven hydrogen evolution

被引：51
|
作者：
Wang, Hong-Yan
Si, Gang
Cao, Wei-Ning
Wang, Wen-Guang
Li, Zhi-Jun
Wang, Feng
Tung, Chen-Ho
Wu, Li-Zhu [1 ]
机构：
[1] Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Photochem Convers & Optoelect Mat, Beijing 100190, Peoples R China
来源：
CHEMICAL COMMUNICATIONS | 2011年 / 47卷 / 29期
基金：
中国国家自然科学基金;
关键词：
ACTIVE-SITE; ELECTRON-TRANSFER; INTRAMOLECULAR ELECTRON; BIOMIMETIC MODEL; PORPHYRIN; LIGAND;
D O I：
10.1039/c1cc12200b
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A novel molecular triad [FeFe]-H(2)ase 1, and its model complexes 2 and 3 have been successfully constructed. The multistep PET and long-lived Fe(I)Fe(0) species were found to be responsible for the better performance of triad 1 than that of 2 with 3 for light-driven H-2 evolution.
引用
收藏
页码：8406 / 8408
页数：3
相关论文
共 50 条
  • [21] Multifunctional Polyoxometalate Platforms for Supramolecular Light-Driven Hydrogen Evolution**
    Maloul, Salam
    van den Borg, Matthias
    Mueller, Carolin
    Zedler, Linda
    Mengele, Alexander K.
    Gaissmaier, Daniel
    Jacob, Timo
    Rau, Sven
    Dietzek-Ivansic, Benjamin
    Streb, Carsten
    CHEMISTRY-A EUROPEAN JOURNAL, 2021, 27 (68) : 16846 - 16852
  • [22] Lanthanum chromite for visible light-driven photocatalytic hydrogen evolution
    Sudrajat, Hanggara
    Hartuti, Sri
    Truong Khang Nguyen
    OPTIK, 2020, 207
  • [23] Catalytic hydrogen evolution from redox complemented [FeFe]-hydrogenase models
    Lansing, James C.
    Camara, James
    Rauchfuss, Thomas
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2013, 246
  • [24] Sonochemical Hydrogen Production as a Potential Interference in Light-Driven Hydrogen Evolution Catalysis
    Roger, Isolda
    Rau, Sven
    Streb, Carsten
    ACS OMEGA, 2020, 5 (33): : 21250 - 21253
  • [25] Iron hydrogenase active site mimics in supramolecular systems aiming for light-driven hydrogen production
    Sun, LC
    Åkermark, B
    Ott, S
    COORDINATION CHEMISTRY REVIEWS, 2005, 249 (15-16) : 1653 - 1663
  • [26] Activating Montmorillonite for Light-Driven Hydrogen Evolution with the Coupling of Fe Species
    Zhang, Wenyan
    Wang, Yihan
    Tao, Weidong
    Guan, Hangmin
    Jiang, Chaoqun
    Tian, Wenjie
    Hao, Lingyun
    ACS APPLIED ENERGY MATERIALS, 2024, 7 (06) : 2504 - 2513
  • [27] Octahedral Tantalum Bromide Clusters as Catalysts for Light-Driven Hydrogen Evolution
    Hernandez, Jhon Sebastian
    Guevara, Daniela
    Shamshurin, Maxim
    Benassi, Enrico
    Sokolov, Maxim N.
    Feliz, Marta
    INORGANIC CHEMISTRY, 2023, 62 (46) : 19060 - 19069
  • [28] Photoinduced Biphasic Hydrogen Evolution: Decamethylosmocene as a Light-Driven Electron Donor
    Ge, Peiyu
    Olaya, Astrid J.
    Scanlon, Micheal D.
    Patir, Imren Hatay
    Vrubel, Heron
    Girault, Hubert H.
    CHEMPHYSCHEM, 2013, 14 (10) : 2308 - 2316
  • [29] Not that innocent - ammonium ions boost homogeneous light-driven hydrogen evolution
    Heiland, Magdalena
    De, Ratnadip
    Rau, Sven
    Dietzek-Ivansic, Benjamin
    Streb, Carsten
    CHEMICAL COMMUNICATIONS, 2022, 58 (29) : 4603 - 4606
  • [30] Optimizing reaction conditions for the light-driven hydrogen evolution in a loop photoreactor
    Li, Pengcheng
    Kowalczyk, Daniel
    Liessem, Johannes
    Elnagar, Mohamed M.
    Mitoraj, Dariusz
    Beranek, Radim
    Ziegenbalg, Dirk
    BEILSTEIN JOURNAL OF ORGANIC CHEMISTRY, 2024, 20 : 74 - 91
12345