The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model

被引:9
作者
Yuan, Guanglu [1 ]
Jiang, Shicheng [1 ]
Wang, Ziwen [1 ]
Hua, Weijie [1 ]
Yu, Chao [1 ]
Jin, Cheng [1 ,2 ]
Lu, Ruifeng [1 ,3 ]
机构
[1] Nanjing Univ Sci & Technol, Dept Appl Phys, Nanjing 210094, Jiangsu, Peoples R China
[2] Chinese Acad Sci, Xian Inst Opt & Precis Mech, State Key Lab Transient Opt & Photon, Xian 710119, Shaanxi, Peoples R China
[3] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China
来源
STRUCTURAL DYNAMICS-US | 2019年 / 6卷 / 05期
基金
中国国家自然科学基金; 美国国家科学基金会;
关键词
DYNAMICS; FANO;
D O I
10.1063/1.5124441
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Based on a multilevel model considering enough bound electronic states of atoms, we theoretically study the role of the transition dipole phase (TDP) in the attosecond transient absorption (ATA) spectrum of helium in intense laser fields. By solving the stationary Schrodinger equation with B-spline basis sets, we first calculate the transition dipole moments with well-defined phases between the bound states. Using the modified multilevel model, we reveal that the TDP plays an important role in determining the spectral structures if two or more paths populate the excited states from the ground state. Our multilevel model with the accurate TDP is convenient to address the origin of atomic ATA spectral structures by freely removing or adding specific electronic states and has been justified by comparing with the ATA spectra via directly solving the time-dependent Schrodinger equation. Hopefully, further incorporating macroscopic propagation into the model will provide indepth physical insights into experimental ATA spectra. (C) 2019 Author(s).
引用
收藏
页数:8
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