Spatio-temporal patterns of air pollution in China from 2015 to 2018 and implications for health risks

被引:160
作者
Kuerban, Mireadili [1 ]
Waili, Yizaitiguli [2 ]
Fan, Fan [1 ]
Liu, Ye [1 ]
Qin, Wei [1 ]
Dore, Anthony J. [3 ]
Peng, Jingjing [1 ]
Xu, Wen [1 ]
Zhang, Fusuo [1 ]
机构
[1] China Agr Univ, Natl Acad Agr Green Dev, Coll Resources & Environm Sci, Key Lab Plant Soil Interact MOE, Beijing 100193, Peoples R China
[2] Xinjiang Univ, Coll Resources & Environm Sci, Urumqi 830046, Peoples R China
[3] Ctr Ecol & Hydrol, Bush Estate, Penicuik EH26 0QB, Midlothian, Scotland
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
Air pollution; Emission control; PM2.5; Ozone; Human health; China; PARTICULATE MATTER PM2.5; PROVINCIAL CAPITAL CITIES; PEARL RIVER DELTA; SURFACE OZONE; ANTHROPOGENIC EMISSIONS; TEMPORAL VARIATIONS; PREMATURE MORTALITY; GASEOUS-POLLUTANTS; DIURNAL-VARIATIONS; NORTHERN CHINA;
D O I
10.1016/j.envpol.2019.113659
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
China has been seriously affected by particulate matter (PM) and gaseous pollutants in the atmosphere. In this study, we systematically analyse the spatio-temporal patterns of PM2.5, PM10, SO2, CO, NO2, and O-3 and the associated health risks, using data collected from 1498 national air quality monitoring sites. An analysis of the averaged data from all the sites indicated that, from 2015 to 2018, annual mean concentrations of PM2.5, PM10, SO2 and CO declined by 3.2 mu g m(-3), 3.7 mu g m(-3), 3.9 mu g m(-3), and 0.1 mg m(-3), respectively. In contrast, those of NO2 and O-3 increased at rates of 0.4 and 3.1 mu g m(-3), respectively. Except for O-3, the annual mean concentrations of all pollutants were generally the highest in North China and lowest in the Tibetan Plateau. The concentrations were generally higher in the north of the country than in the south. In all regions of China, the pollutant concentrations were the highest in winter and lowest in summer, except for O-3, which showed an opposite seasonal pattern. Overall, the seasonal mean concentrations of all the pollutants (except for O-3) significantly decreased between the same seasons in 2018 and 2015, whereas the seasonal mean O-3 concentrations generally significantly increased, and/or remained at stable levels in all four seasons except for winter. Diurnal variations of all pollutants (except for O-3) exhibited a bimodal pattern with peaks between 8:00 and 11:00 a.m. and 9:00 and 12:00 p.m., whereas O-3 exhibited a unimodal pattern with maximum values between 5:00 and 7:00 p.m. No significant differences in the daily mean concentrations of all pollutants were found between weekdays and weekends in all regions, except for PM2.5 and PM10 in Northeast China. In Northwest China and Southeast China, PM2.5 showed stronger correlations with NO2 relative to SO2, suggesting that NOx emission control may be more effective than SO2 emission control for alleviating PM2.5 formation. Compared with 2015, the total PM2.5-attributable mortality, number of respiratory and cardiovascular diseases, and incidence of chronic bronchitis decreased overall by 23.4%-26.9% in 2018. In contrast, for O-3-attributable deaths, there was an increase of 18.9%. Our study not only improves the understanding of the spatial and temporal patterns of air pollutants in China, but also highlights that synchronous control of PM2.5 and O-3 pollution should be implemented to achieve dual benefits in protecting human health. (C) 2019 Elsevier Ltd. All rights reserved.
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页数:12
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