N-Annulated Perylene-Based Push-Pull-Type Sensitizers

被引：44

作者：

Qi, Qingbiao ^{[1
]}

Wang, Xingzhu ^{[2
]}

Fan, Li ^{[2
]}

Zheng, Bin ^{[3
,4
]}

Zeng, Wangdong ^{[1
]}

Luo, Jie ^{[5
]}

Huang, Kuo-Wei ^{[3
,4
]}

Wang, Qing ^{[2
]}

Wu, Jishan ^{[1
,5
]}

机构：

[1] Natl Univ Singapore, Dept Chem, Singapore 117543, Singapore

[2] Natl Univ Singapore, Dept Mat Sci & Engn, NUSNNI NanoCore, Singapore 117576, Singapore

[3] King Abdullah Univ Sci & Technol, KAUST Catalysis Ctr, Thuwal 239556900, Saudi Arabia

[4] King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia

[5] ASTAR, Inst Mat Res & Engn, Singapore 117602, Singapore

来源：

ORGANIC LETTERS | 2015年 / 17卷 / 03期

关键词：

SOLAR-CELLS; ORGANIC-DYES; LIGHT-ABSORPTION; CHARGE-TRANSFER; EFFICIENT; DESIGN; RECOMBINATION; PERFORMANCE; PORPHYRINS; STATES;

D O I：

10.1021/ol503749f

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

Alkoxy-wrapped N-annulated perylene (NP) was synthesized and used as a rigid and coplanar p-linker for three push-pull type metal-free sensitizers QB1-QB3. Their optical and electrochemical properties were tuned by varying the structure of acceptor. These new dyes were applied in Co(II)/(III) based dye-sensitized solar cells, and power conversion efficiency up to 6.95% was achieved, indicating that NP could be used as a new building block for the design of high-performance sensitizers in the future.

引用

页码：724 / 727

页数：4

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