Formation and ordering of topological defect arrays produced by dilatational strain and shear flow in smectic-A liquid crystals

被引:15
作者
Chatterjee, Sourav [1 ]
Anna, Shelley L. [1 ,2 ]
机构
[1] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA
[2] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA
基金
美国国家科学基金会;
关键词
PARABOLIC FOCAL CONICS; UNDULATION INSTABILITY; TEXTURES; LATTICE; PHASE; FILMS;
D O I
10.1103/PhysRevE.85.011701
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
A microscale shear cell is used to study the formation of parabolic focal conic defects in the thermotropic smectic-A liquid crystal 8CB (4-octyl-4'-cyanobiphenyl). Defects are produced by four distinct methods: by the application of dilatational strain alone, by shear flow alone, by dilatational strain and subsequent shear flow, and by the simultaneous application of dilatational strain and shear flow. We confirm that defects originate within the bulk, consistent with the previously suggested undulation instability mechanism. In the presence of a shear flow, we observe that defect formation requires micrometer-level dilatations, whose magnitude depends on the sample thickness. The size and ordering of both disordered and ordered defect arrays is quantified using a pair distribution function. Deviations from the predictions of linear stability theory are observed that have not been reported previously. For example, defects form a square array with greater ordering in the principal flow direction. Ordering due to shear flow does not change the average defect size. It has been shown previously that the principal defect sizes of ordered defects scale differently with sample thickness than the wavelength of the small amplitude undulations. We find that disordered defects show a similar deviation from this predicted wavelength.
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页数:10
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