Optimization of preparation conditions and improvement of stability of Cu/ZnO-based multicomponent catalysts for methanol synthesis from CO2 and H2

被引:61
作者
Wu, JG
Luo, SC
Toyir, J
Saito, M
Takeuchi, M
Watanabe, T
机构
[1] Res Inst Innovat Technol Earth, Tsukuba, Ibaraki 305, Japan
[2] Natl Inst Resources & Environm, Tsukuba, Ibaraki 305, Japan
[3] Res Inst Innovat Technol Earth, Kizu, Kyoto 61902, Japan
关键词
CO2 hydrogenation into methanol; Cu/ZnO-based catalyst; preparation conditions; stability improvement;
D O I
10.1016/S0920-5861(98)00218-1
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
The operation conditions for preparing a Cu/ZnO-based multicomponent catalyst by a coprecipitation method were optimized. The temperature during coprecipitation should be less than 313 K, and the removal of Na from the catalyst by washing the precipitates is most important. Furthermore, a small amount of silica added to the catalyst greatly improved its long-term stability in methanol synthesis from CO2 and H-2. (C) 1998 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:215 / 220
页数:6
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