Compensatory effect of biomass burning on black carbon concentrations during COVID-19 lockdown at a high-altitude station in SW India

被引:8
作者
Mukherjee, Subrata [1 ,2 ]
Verma, Aastha [3 ]
Meena, Guman Singh [1 ]
Kodoli, Sandeep [1 ]
Buchunde, Pallavi [1 ,2 ]
Aslam, Mohammed Yusuff [1 ]
Patil, Rohit Dilip [1 ]
Panicker, Abhilash [1 ]
Safai, Pramod Digambar [1 ]
Pandithurai, Govindan [1 ]
机构
[1] Minist Earth Sci, Indian Inst Trop Meteorol, Pune, India
[2] Savitribai Phule Pune Univ, Pune, India
[3] Cent Univ South Bihar, Patna, India
关键词
Black carbon; Source apportionment; AAE; Radiative forcing; Brown carbon; ABSORPTION ANGSTROM EXPONENT; BROWN CARBON; LIGHT-ABSORPTION; SOURCE APPORTIONMENT; AEROSOL MASS; SEASONAL VARIABILITY; CHEMICAL-COMPOSITION; OPTICAL-PROPERTIES; ORGANIC AEROSOLS; WESTERN-GHATS;
D O I
10.1016/j.apr.2022.101566
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The characteristics of black carbon (BC) aerosols, their sources, and their impact on atmospheric radiative forcing were extensively studied during the COVID-19 lockdown (28th March-31st May 2020) at a high-altitude rural site over the Western Ghats in southwest India. BC concentration and the contribution of BC originating from biomass burning (BCbb) estimated from the aethalometer model during the lockdown period were compared with the same periods in 2017 and 2018 and with the pre-lockdown period (1st February to March 20, 2020). BC concentrations were 44, 19, and 17% lower during the lockdown period compared with the prelockdown periods of 2020 and similar periods (28th March to 31st May) of 2017 and 2018, respectively. BCbb contributed similar to 50% to total BC during the lockdown period of 2020 and compensated for the decrease in BC concentration due to lower traffic emissions. The characteristics of light-absorbing organic carbon (brown carbon; BrC) absorption at 370 nm were evaluated during the lockdown and the pre-lockdown periods of 2020, 2017, and 2018. The BrC was estimated to be the highest during the lockdown period of 2020. Finally, atmospheric radiative forcing was calculated using the mean BC concentration during the pre-lockdown, lockdown, and similar periods (28th March to 31st May) of 2017 and 2018.
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页数:10
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共 77 条
[1]   O/C and OM/OC ratios of primary, secondary, and ambient organic aerosols with high-resolution time-of-flight aerosol mass spectrometry [J].
Aiken, Allison C. ;
Decarlo, Peter F. ;
Kroll, Jesse H. ;
Worsnop, Douglas R. ;
Huffman, J. Alex ;
Docherty, Kenneth S. ;
Ulbrich, Ingrid M. ;
Mohr, Claudia ;
Kimmel, Joel R. ;
Sueper, Donna ;
Sun, Yele ;
Zhang, Qi ;
Trimborn, Achim ;
Northway, Megan ;
Ziemann, Paul J. ;
Canagaratna, Manjula R. ;
Onasch, Timothy B. ;
Alfarra, M. Rami ;
Prevot, Andre S. H. ;
Dommen, Josef ;
Duplissy, Jonathan ;
Metzger, Axel ;
Baltensperger, Urs ;
Jimenez, Jose L. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008, 42 (12) :4478-4485
[2]   Impact of lockdown-related reduction in anthropogenic emissions on aerosol characteristics in the megacity, Bengaluru [J].
Ajay, A. ;
Moorthy, K. Krishna ;
Satheesh, S. K. ;
Ilavazhagan, G. .
CURRENT SCIENCE, 2021, 120 (02) :287-295
[3]   Identification of the mass spectral signature of organic aerosols from wood burning emissions [J].
Alfarra, M. Rami ;
Prevot, Andre S. H. ;
Szidat, Sonke ;
Sandradewi, Jisca ;
Weimer, Silke ;
Lanz, Valentin A. ;
Schreiber, Daniel ;
Mohr, Martin ;
Baltensperger, Urs .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2007, 41 (16) :5770-5777
[4]   Black carbon or brown carbon?: The nature of light-absorbing carbonaceous aerosols [J].
Andreae, M. O. ;
Gelencser, A. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2006, 6 :3131-3148
[5]   Radiative Impacts of Aerosols During COVID-19 Lockdown Period Over the Indian Region [J].
Bhawar, Rohini L. ;
Fadnavis, Suvarna ;
Kumar, Vinay ;
Rahul, P. R. C. ;
Sinha, Tushar ;
Lolli, Simone .
FRONTIERS IN ENVIRONMENTAL SCIENCE, 2021, 9
[6]   Bounding the role of black carbon in the climate system: A scientific assessment [J].
Bond, T. C. ;
Doherty, S. J. ;
Fahey, D. W. ;
Forster, P. M. ;
Berntsen, T. ;
DeAngelo, B. J. ;
Flanner, M. G. ;
Ghan, S. ;
Kaercher, B. ;
Koch, D. ;
Kinne, S. ;
Kondo, Y. ;
Quinn, P. K. ;
Sarofim, M. C. ;
Schultz, M. G. ;
Schulz, M. ;
Venkataraman, C. ;
Zhang, H. ;
Zhang, S. ;
Bellouin, N. ;
Guttikunda, S. K. ;
Hopke, P. K. ;
Jacobson, M. Z. ;
Kaiser, J. W. ;
Klimont, Z. ;
Lohmann, U. ;
Schwarz, J. P. ;
Shindell, D. ;
Storelvmo, T. ;
Warren, S. G. ;
Zender, C. S. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2013, 118 (11) :5380-5552
[7]   Seasonal abundances of primary and secondary carbonaceous aerosols at a high-altitude station in the Western Ghat Mountains, India [J].
Buchunde, P. S. ;
Safai, P. D. ;
Mukherjee, S. ;
Raju, M. P. ;
Meena, G. S. ;
Sonbawne, S. M. ;
Dani, K. K. ;
Pandithurai, G. .
AIR QUALITY ATMOSPHERE AND HEALTH, 2022, 15 (02) :209-220
[8]   The atmospheric lifetime of black carbon [J].
Cape, J. N. ;
Coyle, M. ;
Dumitrean, P. .
ATMOSPHERIC ENVIRONMENT, 2012, 59 :256-263
[9]   Brown carbon in tar balls from smoldering biomass combustion [J].
Chakrabarty, R. K. ;
Moosmueller, H. ;
Chen, L. -W. A. ;
Lewis, K. ;
Arnott, W. P. ;
Mazzoleni, C. ;
Dubey, M. K. ;
Wold, C. E. ;
Hao, W. M. ;
Kreidenweis, S. M. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (13) :6363-6370
[10]   Light absorption by organic carbon from wood combustion [J].
Chen, Y. ;
Bond, T. C. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (04) :1773-1787